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  Zirconium‐Assisted Activation of Palladium To Boost Syngas Production by Methane Dry Reforming

Köpfle, N., Götsch, T., Grünbacher, M., Carbonio, E., Hävecker, M., Knop-Gericke, A., et al. (2018). Zirconium‐Assisted Activation of Palladium To Boost Syngas Production by Methane Dry Reforming. Angewandte Chemie International Edition, 57(44), 14613-14618. doi:10.1002/anie.201807463.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0002-8934-9 Version Permalink: https://hdl.handle.net/21.11116/0000-0009-87AF-A
Genre: Journal Article

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K-pfle_et_al-2018-Angewandte_Chemie_International_Edition.pdf (Publisher version), 3MB
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K-pfle_et_al-2018-Angewandte_Chemie_International_Edition.pdf
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2018
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http://creativecommons.org/licenses/by/4.0/

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 Creators:
Köpfle, Norbert1, Author
Götsch, Thomas1, Author
Grünbacher, Matthias1, Author
Carbonio, Emilia2, 3, Author           
Hävecker, Michael2, Author           
Knop-Gericke, Axel2, Author           
Schlicker, Lukas4, Author
Doran, Andrew5, Author
Kober, Delf4, Author
Gurlo, Aleksander4, Author
Penner, Simon1, Author
Klötzer, Bernhard1, Author
Affiliations:
1Institute of Physical Chemistry, University of Innsbruck, Innrain 52 c, A-6020 Innsbruck, Austria, ou_persistent22              
2Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              
3Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, BESSY II, Albert-Einstein-Straße 15, 12489 Berlin, Germany, ou_persistent22              
4Fachgebiet Keramische Werkstoffe, Institut für Werkstoffwissenschaften und -technologien, Technische Universität Berlin, Hardenbergstr. 40, D-10623 Berlin, Germany, ou_persistent22              
5Advanced Light Source, Beamline 12.2.2., Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA, ou_persistent22              

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 Abstract: C‐saturated Pd0 nanoparticles with an extended phase boundary to ZrO2 evolve from a Pd0Zr0 precatalyst under CH4 dry reforming conditions. This highly active catalyst state fosters bifunctional action: CO2 is efficiently activated at oxidic phase boundary sites and PdxC provides fast supply of C‐atoms toward the latter.

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Language(s): eng - English
 Dates: 2018-06-282018-10-232018-10-26
 Publication Status: Issued
 Pages: 6
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/anie.201807463
 Degree: -

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Project name : CALIPSOplus - Convenient Access to Light Sources Open to Innovation, Science and to the World
Grant ID : 730872
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)

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Title: Angewandte Chemie International Edition
  Other : Angew. Chem. Int. Ed.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: 6 Volume / Issue: 57 (44) Sequence Number: - Start / End Page: 14613 - 14618 Identifier: ISSN: 1433-7851
CoNE: https://pure.mpg.de/cone/journals/resource/1433-7851