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  Control and imaging of single-molecule spectral dynamics using a nano-electrode

Gerhardt, I., Wrigge, G., & Sandoghdar, V. (2009). Control and imaging of single-molecule spectral dynamics using a nano-electrode. Molecular Physics, 107: PII 914467980, pp. 1975-1979. doi:10.1080/00268970903188358.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0002-9A8F-0 Version Permalink: https://hdl.handle.net/21.11116/0000-0007-953F-B
Genre: Journal Article

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 Creators:
Gerhardt, I.1, Author
Wrigge, G.1, Author
Sandoghdar, Vahid2, Author           
Affiliations:
1external, ou_persistent22              
2External Organizations, ou_persistent22              

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 Abstract: We study the influence of a scanning nano-electrode on the fluorescence excitation spectra of single terrylene molecules embedded in thin p-terphenyl films at cryogenic temperatures. We show that applied voltages of less than 10 V can result in reversible Stark shifts of up to 100 times and a linewidth increase greater than 10 times the natural linewidth. We discuss the potential of our experimental scheme for the direct imaging of individual two-level systems in the nanometer vicinity of single molecules.

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Language(s): eng - English
 Dates: 2009
 Publication Status: Published online
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: -
 Identifiers: DOI: 10.1080/00268970903188358
 Degree: -

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Title: Molecular Physics
  Other : Mol. Phys.
Source Genre: Journal
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Publ. Info: London : Taylor & Francis
Pages: - Volume / Issue: 107 Sequence Number: PII 914467980 Start / End Page: 1975 - 1979 Identifier: ISSN: 0026-8976
CoNE: https://pure.mpg.de/cone/journals/resource/954925264211