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  Stimulated resonant inelastic x-ray scattering with chirped, broadband pulses

Hollstein, M., & Rohringer, N. (2019). Stimulated resonant inelastic x-ray scattering with chirped, broadband pulses. Physical Review A, 99(1): 013425. doi:10.1103/PhysRevA.99.013425.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0002-D984-4 Version Permalink: http://hdl.handle.net/21.11116/0000-0004-8FBE-6
Genre: Journal Article

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PhysRevA.99.013425.pdf (Publisher version), 2MB
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© American Physical Society

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https://arxiv.org/abs/1811.04292 (Preprint)
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https://dx.doi.org/10.1103/PhysRevA.99.013425 (Publisher version)
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 Creators:
Hollstein, M.1, Author
Rohringer, N.1, 2, 3, Author              
Affiliations:
1Quantum Optics with X-Rays, Independent Research Groups, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938291              
2Center for Free-Electron Laser Science, DESY, ou_persistent22              
3Department of Physics, University of Hamburg, ou_persistent22              

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 Abstract: We present an approach for initiating and tracing ultrafast electron dynamics in core-excited atoms, molecules, and solids. The approach is based on stimulated resonant inelastic x-ray scattering induced by a single, chirped, broadband XUV or x-ray pulse. A first interaction with this pulse prepares a core-excited state wave packet by resonant core-excitation. A second interaction with the pulse at a later time induces the transition to valence-excited states, which is associated with stimulated emission. The preparation of the core-excited wave packet and the transition from the core-excited states to the valence-excited states occur at distinct chirp-dependent times. As a consequence, the stimulated emission carries information about the time evolution of the core-excited state wave packet.

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Language(s): eng - English
 Dates: 2018-11-102018-04-242019-01-182019-01-18
 Publication Status: Published in print
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 Table of Contents: -
 Rev. Method: Peer
 Identifiers: arXiv: 1811.04292
DOI: 10.1103/PhysRevA.99.013425
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Title: Physical Review A
  Other : Physical Review A: Atomic, Molecular, and Optical Physics
  Other : Phys. Rev. A
Source Genre: Journal
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Publ. Info: New York, NY : American Physical Society
Pages: - Volume / Issue: 99 (1) Sequence Number: 013425 Start / End Page: - Identifier: ISSN: 1050-2947
CoNE: https://pure.mpg.de/cone/journals/resource/954925225012_2