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  Grafting Polymers onto Carbon Nitride via Visible-Light-Induced Photofunctionalization

Cao, Q., Kumru, B., Antonietti, M., & Schmidt, B. V. K. J. (2019). Grafting Polymers onto Carbon Nitride via Visible-Light-Induced Photofunctionalization. Macromolecules, 52(13), 4989-4996. doi:10.1021/acs.macromol.9b00894.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0003-E457-A Version Permalink: http://hdl.handle.net/21.11116/0000-0004-5D71-5
Genre: Journal Article

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 Creators:
Cao, Qian1, Author              
Kumru, Baris1, Author              
Antonietti, Markus2, Author              
Schmidt, Bernhard V. K. J.1, Author              
Affiliations:
1Bernhard Schmidt, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2149676              
2Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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 Abstract: Metal-free graphitic carbon nitride (g-CN) has attracted significant attention recently due to its multiple applications, such as photocatalysis, energy storage and conversion, and biomaterials, albeit formation of g-CN films is challenging. Herein, a “grafting to” route to graft polymer brushes onto g-CN via visible-light irradiation is described. Afterward, g-CN/polymer films can be obtained through spin coating on glass substrates. As such, the present material provides an improved process toward further application of g-CN in thin films. Moreover, an improved dispersibility in organic solvent was realized after grafting and functional groups (such as epoxides) were introduced to g-CN. Subsequently, the epoxy groups were utilized for further functionalization to adjust the surface polarity.

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 Dates: 2019-06-202019
 Publication Status: Published in print
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 Identifiers: DOI: 10.1021/acs.macromol.9b00894
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Title: Macromolecules
  Other : Macromolecules
Source Genre: Journal
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Publ. Info: Washington, D.C. : American Chemical Society
Pages: - Volume / Issue: 52 (13) Sequence Number: - Start / End Page: 4989 - 4996 Identifier: ISSN: 0024-9297