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  Direct observation of interatomic Coulombic decay and subsequent ion-atom scattering in helium nanodroplets

Wiegandt, F., Trinter, F., Henrichs, K., Metz, D., Pitzer, M., Waitz, M., et al. (2019). Direct observation of interatomic Coulombic decay and subsequent ion-atom scattering in helium nanodroplets. Physical Review A, 100(2): 022707. doi:10.1103/PhysRevA.100.022707.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0004-8B3A-F Version Permalink: http://hdl.handle.net/21.11116/0000-0004-8C30-8
Genre: Journal Article

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PhysRevA.100.022707.pdf (Publisher version), 2MB
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PhysRevA.100.022707.pdf
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 Creators:
Wiegandt, F.1, 2, Author
Trinter, Florian1, 3, 4, Author
Henrichs, K.1, Author
Metz, D.1, Author
Pitzer, M.5, Author
Waitz, M.1, Author
Maalouf, E. Jabbour al6, Author
Janke, C.1, Author
Rist, J.1, Author
Wechselberger, N.1, Author
Miteva, T.7, Author
Kazandjian, S.7, Author
Schöffler, M.1, Author
Sisourat, N.7, Author
Jahnke, T.1, Author
Dörner, R.1, Author
Affiliations:
1Institut für Kernphysik, Goethe Universität, Max-von-Laue-Strasse 1, D-60438 Frankfurt, Germany, ou_persistent22              
2Clarendon Laboratory, Department of Physics, University of Oxford, Oxford OX1 3PU, United Kingdom, ou_persistent22              
3Deutsches Elektronen-Synchrotron (DESY), FS-PETRA-S, Notkestrasse 85, D-22607 Hamburg, Germany, ou_persistent22              
4Molecular Physics, Fritz Haber Institute, Max Planck Society, Berlin, DE, ou_634545              
5Department of Chemical and Biological Physics, Weizmann Institute of Science, P.O. Box 26, 76100 Rehovot, Israel, ou_persistent22              
6Institut für Ionenphysik und Angewandte Physik, Universität Innsbruck, Technikerstrasse 25, 6020 Innsbruck, Austria, ou_persistent22              
7Sorbonne Université, CNRS, Laboratoire de Chimie Physique Matière et Rayonnement, UMR 7614, F-75005 Paris, France, ou_persistent22              

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 Abstract: We report on the experimental observation of interatomic Coulombic decay (ICD) in pure 4He nanoclusters of mean sizes between N ∼ 5000 and 30 000 and the subsequent scattering of energetic He+ fragments inside the neutral cluster by using cold target recoil ion momentum spectroscopy. ICD is induced in He clusters by using vacuum ultraviolet light of hν=67eV from the BESSY II synchrotron. The electronic decay creates two neighboring ions in the cluster at a well-defined distance. The measured fragment energies and angular correlations show that a main energy loss mechanism of these ions inside the cluster is a single hard binary collision with one atom of the cluster.

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Language(s): eng - English
 Dates: 2019-06-242019-08-262019-08
 Publication Status: Published in print
 Pages: 6
 Publishing info: -
 Table of Contents: -
 Rev. Method: Peer
 Identifiers: DOI: 10.1103/PhysRevA.100.022707
 Degree: -

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Title: Physical Review A
  Other : Physical Review A: Atomic, Molecular, and Optical Physics
  Other : Phys. Rev. A
Source Genre: Journal
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Publ. Info: New York, NY : American Physical Society
Pages: - Volume / Issue: 100 (2) Sequence Number: 022707 Start / End Page: - Identifier: ISSN: 1050-2947
CoNE: https://pure.mpg.de/cone/journals/resource/954925225012_2