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  Oxysulfide semiconductors for photocatalytic overall water splitting with visible light

Zhang, G., & Wang, X. (2019). Oxysulfide semiconductors for photocatalytic overall water splitting with visible light. Angewandte Chemie, International Edition, 58(44), 15580-15582. doi:10.1002/anie.201909669.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0004-E4FE-D Version Permalink: http://hdl.handle.net/21.11116/0000-0004-E4FF-C
Genre: Journal Article

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 Creators:
Zhang, Guigang1, Author              
Wang, Xinchen, Author
Affiliations:
1Aleksandr Savateev, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2421702              

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Free keywords: charge separation, orbital hybridization, oxysulfides, photocatalyst durability, surface engineering
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Language(s): eng - English
 Dates: 2019-09-302019
 Publication Status: Published in print
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 Table of Contents: Photocatalytic overall water splitting by sulfide‐based materials is a great challenge because of the poor resilience of such materials against hole oxidation. In a recent study, Domen and co‐workers developed an innovative strategy to stabilize sulfide‐based photocatalysts by hybridizing S 3p with O 2p orbitals to produce oxysulfides in which S2− is stable. Further surface engineering of the oxysulfides with dual co‐catalysts promoted charge separation and interface transfer, thus reducing the charge build‐up that inhibits photocorrosion. The pH value of the reaction mixture is a critical consideration for achieving efficient stoichiometric H2 and O2 evolution by these oxysulfide photocatalysts.
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 Identifiers: DOI: 10.1002/anie.201909669
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Title: Angewandte Chemie, International Edition
  Abbreviation : Angew. Chem., Int. Ed.
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 58 (44) Sequence Number: - Start / End Page: 15580 - 15582 Identifier: ISSN: 1433-7851