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  Electronic Decay of Singly Charged Ground-State Ions by Charge Transfer via van der Waals Bonds

Hans, A., Miteva, T., Holzapfel, X., Ozga, C., Schmidt, P., Otto, H., et al. (2019). Electronic Decay of Singly Charged Ground-State Ions by Charge Transfer via van der Waals Bonds. Physical Review Letters, 123(21): 312001. doi:10.1103/PhysRevLett.123.213001.

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 Creators:
Hans, Andreas1, 2, Author
Miteva, Tsveta3, Author
Holzapfel, Xaver1, Author
Ozga, Christian1, Author
Schmidt, Philipp1, Author
Otto, Huda1, Author
Hartmann, Gregor1, Author
Richter, Clemens4, Author
Sisourat, Nicolas3, Author
Ehresmann, Arno1, Author
Gokhberg, Kirill5, Author
Hergenhahn, U.4, 6, Author           
Knie, André1, Author
Affiliations:
1Universität Kassel, Institut für Physik und CINSaT, Heinrich-Plett-Str. 40, D-34132 Kassel, Germany, ou_persistent22              
2Nano and Molecular Systems Research Unit, Faculty of Science, University of Oulu, P.O. Box 3000, 90014 Oulu, Finland, ou_persistent22              
3Laboratoire de Chimie Physique Matière et Rayonnement, UMR 7614, Sorbonne Université, CNRS, F-75005 Paris, France, ou_persistent22              
4Leibniz-Institut für Oberflächenmodifizierung (IOM), Permoserstr. 15, D-04318 Leipzig, Germany, ou_persistent22              
5Physikalisch-Chemisches Institut, Universität Heidelberg, Im Neuenheimer Feld 229, D-69120 Heidelberg, Germany, ou_persistent22              
6Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              

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 Abstract: We report the observation of the radiative decay of singly charged noble gas ground-state ions embedded in heterogeneous van der Waals clusters. Electron-photon coincidence spectroscopy and dispersed photon spectroscopy are applied to identify the radiative charge transfer from Kr atoms to a Ne+2 dimer, which forms after single valence photoionization of Ne atoms at the surface of a NeKr cluster. This mechanism might be a fundamental decay process of ionized systems in an environment.

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Language(s): eng - English
 Dates: 2019-06-122019-11-192019-11-22
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.123.213001
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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 123 (21) Sequence Number: 312001 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1