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  Photon-Momentum-Induced Molecular Dynamics in Photoionization of N2 at hν = 40 keV

Kircher, M., Rist, J., Trinter, F., Grundmann, S., Waitz, M., Melzer, N., et al. (2019). Photon-Momentum-Induced Molecular Dynamics in Photoionization of N2 at hν = 40 keV. Physical Review Letters, 123(19): 193001. doi:10.1103/PhysRevLett.123.193001.

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PhysRevLett.123.193001.pdf (Publisher version), 642KB
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PhysRevLett.123.193001.pdf
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 Creators:
Kircher, M.1, Author
Rist, J.1, Author
Trinter, Florian2, 3, Author           
Grundmann, S.1, Author
Waitz, M.1, Author
Melzer, N.1, Author
Vela-Perez, I.1, Author
Mletzko, T.1, Author
Pier, A.1, Author
Strenger, N.1, Author
Siebert, J.1, Author
Janssen, R.1, Author
Honkimäki, V.4, Author
Drnec, J.4, Author
Demekhin, Ph. V.5, Author
Schmidt, L. Ph. H.1, Author
Schöffler, M. S.1, Author
Jahnke, T.1, Author
Dörner, R.1, Author
Affiliations:
1Institut für Kernphysik, Johann Wolfgang Goethe Universität, Max-von-Laue-Strasse 1, 60438 Frankfurt, Germany, ou_persistent22              
2FS-PETRA-S, Deutsches Elektronen-Sychrotron (DESY), Notkestrasse 85, 22607 Hamburg, Germany, ou_persistent22              
3Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
4ESRF, 6 Rue Jules Horowitz, BP 220, 38043 Grenoble Cedex 9, France, ou_persistent22              
5Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Strasse 40, 34132 Kassel, Germany, ou_persistent22              

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 Abstract: We investigate K-shell ionization of N2 at 40 keV photon energy. Using a cold target recoil ion momentum spectroscopy reaction microscope, we determine the vector momenta of the photoelectron, the Auger electron, and both N+ fragments. These fully differential data show that the dissociation process of the N2+2 ion is significantly modified not only by the recoil momentum of the photoelectron but also by the photon momentum and the momentum of the emitted Auger electron. We find that the recoil energy introduced by the photon and the photoelectron momentum is partitioned with a ratio of approximately 30∶70 between the Auger electron and fragment ion kinetic energies, respectively. We also observe that the photon momentum induces an additional rotation of the molecular ion.

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Language(s): eng - English
 Dates: 2019-07-022019-11-052019-11-08
 Publication Status: Issued
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.123.193001
 Degree: -

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Title: Physical Review Letters
  Alternative Title : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 123 (19) Sequence Number: 193001 Start / End Page: - Identifier: n.a.: /journals/resource/954925433406_1