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  Detection of the 5p-4f orbital crossing and its optical clock transition in Pr9+

Bekker, H., Borschevsky, A., Harman, Z., Keitel, C. H., Pfeifer, T., Schmidt, P. O., et al. (2019). Detection of the 5p-4f orbital crossing and its optical clock transition in Pr9+. Nature Communications, 10: 5651. doi:10.1038/s41467-019-13406-9.

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1910.09010.pdf (Preprint), 719KB
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MPIK-Pressemitteilung: Hochgeladenes Ion bahnt den Weg zu neuer Physik
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 Creators:
Bekker, Hendrik1, Author           
Borschevsky , A., Author
Harman, Z.2, Author           
Keitel, C. H.2, Author           
Pfeifer, T.1, Author           
Schmidt , P. O., Author
Crespo López Urrutia, J. R.1, Author           
Berengut, J. C., Author
Affiliations:
1Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society, ou_2025284              
2Division Prof. Dr. Christoph H. Keitel, MPI for Nuclear Physics, Max Planck Society, ou_904546              

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Free keywords: Physics, Atomic Physics, physics.atom-ph
 MPINP: Research group Z. Harman – Division C. H. Keitel
 Abstract: Recent theoretical works have proposed atomic clocks based on narrow optical
transitions in highly charged ions. The most interesting candidates for
searches of new physics are those which occur at rare orbital crossings where
the shell structure of the periodic table is reordered. There are only three
such crossings expected to be accessible in highly charged ions, and hitherto
none have been observed as both experiment and theory have proven difficult. In
this work we observe an orbital crossing in highly charged ions for the first
time, in a system chosen to be tractable from both sides: Pr9+. We present
electron beam ion trap measurements of its spectra, including the
inter-configuration lines that reveal the sought-after crossing. The proposed
nHz-wide clock line, found to be at 452.334(1) nm, proceeds through hyperfine
admixture of its upper state with an E2-decaying level. With state-of-the-art
calculations we show that it has a very high sensitivity to new physics and
extremely low sensitivity to external perturbations, making it a unique
candidate for proposed precision studies.

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 Dates: 2019-12-11
 Publication Status: Published online
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 Rev. Type: Peer
 Identifiers: arXiv: 1910.09010
DOI: 10.1038/s41467-019-13406-9
 Degree: -

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Title: Nature Communications
  Abbreviation : Nat. Commun.
Source Genre: Journal
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Publ. Info: London : Nature Publishing Group
Pages: - Volume / Issue: 10 Sequence Number: 5651 Start / End Page: - Identifier: ISSN: 2041-1723
CoNE: https://pure.mpg.de/cone/journals/resource/2041-1723