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  Visible-light flow reactor packed with porous carbon nitride for aerobic substrate oxidations

Bajada, M., Vijeta, A., Savateev, A., Zhang, G., Howe, D., & Reisner, E. (2020). Visible-light flow reactor packed with porous carbon nitride for aerobic substrate oxidations. ACS Applied Materials and Interfaces, 12(7), 8176-8182. doi:10.1021/acsami.9b19718.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0005-9BFF-E Version Permalink: http://hdl.handle.net/21.11116/0000-0005-E268-7
Genre: Journal Article

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 Creators:
Bajada, Mark, Author
Vijeta, Arjun, Author
Savateev, Aleksandr1, Author              
Zhang, Guigang1, Author              
Howe, Duncan, Author
Reisner, Erwin, Author
Affiliations:
1Aleksandr Savateev, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2421702              

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Free keywords: photocatalysis; flow chemistry; aerobic oxidation; carbon nitride; green chemistry
 Abstract: A triphasic photocatalytic reactor employing a mesoporous carbon nitride photocatalyst and aerobic O2 was assembled to operate under continuous flow conditions. This reactor design allows for facile downstream processing and reusability in multiple flow cycles. The selective aerobic oxidation of alcohols and amines was chosen to demonstrate the applicability and performance advantage of this flow approach compared to conventional batch photochemistry. This precious-metal-free photocatalytic flow system operates under benign reaction conditions (visible light, low pressure, and mild temperature) and will stimulate the exploration of other oxidative reactions in a sustainable, scalable, and affordable manner.

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Language(s): eng - English
 Dates: 2020-01-212020
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Method: -
 Identifiers: DOI: 10.1021/acsami.9b19718
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Title: ACS Applied Materials and Interfaces
  Abbreviation : ACS Appl. Mater. Interfaces
Source Genre: Journal
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Publ. Info: Washington, DC : American Chemical Society
Pages: - Volume / Issue: 12 (7) Sequence Number: - Start / End Page: 8176 - 8182 Identifier: ISSN: 1944-8244