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  Interplay of porosity, wettability, and redox activity as determining factors for lithium-organic electrochemical energy storage using biomolecules

Ilic, I., Perovic, M., & Liedel, C. (2020). Interplay of porosity, wettability, and redox activity as determining factors for lithium-organic electrochemical energy storage using biomolecules. ChemSusChem, 13(7), 1856-1863. doi:10.1002/cssc.201903156.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0005-A6BD-B Version Permalink: http://hdl.handle.net/21.11116/0000-0006-1FF1-8
Genre: Journal Article

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 Creators:
Ilic, Ivan1, Author              
Perovic, Milena2, Author              
Liedel, Clemens1, Author              
Affiliations:
1Clemens Liedel, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2288694              
2Martin Oschatz, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2364733              

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Free keywords: energy storage, guaiacol, wettability, redox activity, vanillin
 Abstract: While several recent publications describe cathodes for electrochemical energy storage materials made from regrown biomass in aqueous electrolytes, their transfer to lithium-organic batteries is challenging. In order to gain a deeper understanding, we therefore investigate influences on charge storage in model systems based on biomass-derived, redox-active compounds and comparable structures. Hybrid materials from these model polymers and porous carbon are compared in order to precisely determine causes of exceptional capacity in lithium-organic systems. It is found that besides redox activity especially wettability greatly influences capacity of the composites. Furthermore, in addition to bio-derived molecules with catechol functionalities, which are commonly described as redox-active species in lithium-bioorganic systems, this manuscript further describes guaiacol groups as a promising alternative for the first time and compares performance of respective compounds.

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Language(s): eng - English
 Dates: 2020-02-052020
 Publication Status: Published in print
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 Identifiers: DOI: 10.1002/cssc.201903156
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Title: ChemSusChem
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 13 (7) Sequence Number: - Start / End Page: 1856 - 1863 Identifier: ISSN: 1864-5631