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  Interplay of porosity, wettability, and redox activity as determining factors for lithium-organic electrochemical energy storage using biomolecules

Ilic, I., Perovic, M., & Liedel, C. (2020). Interplay of porosity, wettability, and redox activity as determining factors for lithium-organic electrochemical energy storage using biomolecules. ChemSusChem, 13(7), 1856-1863. doi:10.1002/cssc.201903156.

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 Urheber:
Ilic, Ivan1, Autor           
Perovic, Milena2, Autor           
Liedel, Clemens1, Autor           
Affiliations:
1Clemens Liedel, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2288694              
2Martin Oschatz, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2364733              

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Schlagwörter: energy storage, guaiacol, wettability, redox activity, vanillin
 Zusammenfassung: While several recent publications describe cathodes for electrochemical energy storage materials made from regrown biomass in aqueous electrolytes, their transfer to lithium-organic batteries is challenging. In order to gain a deeper understanding, we therefore investigate influences on charge storage in model systems based on biomass-derived, redox-active compounds and comparable structures. Hybrid materials from these model polymers and porous carbon are compared in order to precisely determine causes of exceptional capacity in lithium-organic systems. It is found that besides redox activity especially wettability greatly influences capacity of the composites. Furthermore, in addition to bio-derived molecules with catechol functionalities, which are commonly described as redox-active species in lithium-bioorganic systems, this manuscript further describes guaiacol groups as a promising alternative for the first time and compares performance of respective compounds.

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Sprache(n): eng - English
 Datum: 2020-02-052020
 Publikationsstatus: Erschienen
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 Identifikatoren: DOI: 10.1002/cssc.201903156
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Titel: ChemSusChem
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: Weinheim : Wiley-VCH
Seiten: - Band / Heft: 13 (7) Artikelnummer: - Start- / Endseite: 1856 - 1863 Identifikator: ISSN: 1864-5631