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  Revealing Hidden Orbital Pseudospin Texture with Time-Reversal Dichroism in Photoelectron Angular Distributions

Beaulieu, S., Schusser, J., Dong, S., Schüler, M., Pincelli, T., Dendzik, M. R., et al. (2020). Revealing Hidden Orbital Pseudospin Texture with Time-Reversal Dichroism in Photoelectron Angular Distributions. Physical Review Letters, 125(21): 216404. doi:10.1103/PhysRevLett.125.216404.

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 Urheber:
Beaulieu, Samuel1, Autor           
Schusser, Jakub2, 3, Autor
Dong, Shuo1, Autor           
Schüler, M.4, Autor
Pincelli, Tommaso1, Autor           
Dendzik, Maciej Ramon1, 5, Autor           
Maklar, Julian1, Autor           
Neef, Alexander1, Autor           
Ebert, Hubert6, Autor
Hricovini, Karol2, 7, Autor
Wolf, Martin1, Autor           
Braun, Jürgen6, Autor
Rettig, Laurenz1, Autor           
Minár, Jan2, Autor
Ernstorfer, Ralph1, Autor           
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
2Laboratoire de Physique des Matériaux et Surfaces, CY Cergy Paris Université, 95031 Cergy-Pontoise, France, ou_persistent22              
3New Technologies-Research Center, University of West Bohemia, 30614 Pilsen, Czech Republic, ou_persistent22              
4Stanford Institute for Materials and Energy Sciences (SIMES), SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA, ou_persistent22              
5Department of Applied Physics, KTH Royal Institute of Technology, Electrum 229, SE-16440, Stockholm, Kista, Sweden, ou_persistent22              
6Department Chemie, Ludwig-Maximilians-Universität München, Butenandtstrasse 11, 81377 München, Germany, ou_persistent22              
7LIDYL, CEA, CNRS (UMR 9222), Université Paris-Saclay, CEA Saclay, F-91191, Gif-sur-Yvette Cedex, France, ou_persistent22              

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Schlagwörter: Condensed Matter, Materials Science, cond-mat.mtrl-sci, Condensed Matter, cond-mat.other
 Zusammenfassung: We performed angle-resolved photoemission spectroscopy (ARPES) of bulk
2H-WSe$_2$ for different crystal orientations linked to each other by
time-reversal symmetry. We introduce a new observable called time-reversal
dichroism, which quantifies the modulation of the photoemission intensity upon
effective time-reversal operation. We demonstrate that the hidden
orbital-texture of the crystal's electronic structure leaves its imprint onto
the time-reversal dichroism, due to multiple orbitals interference effects in
photoemission. Our experimental results are in quantitative agreement with
state-of-the-art fully relativistic calculations performed using the one-step
model of photoemission. While spin-resolved ARPES probes the spin component of
entangled spin-orbital texture in multiorbital systems, we demonstrate that
time-reversal dichroism is sensitive to its orbital-texture counterpart.

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Sprache(n): eng - English
 Datum: 2020-06-022020-08-272020-06-022020-10-132020-11-202020-11-20
 Publikationsstatus: Erschienen
 Seiten: 6
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Art des Abschluß: -

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Projektname : FLATLAND - Electron-lattice-spin correlations and many-body phenomena in 2D semiconductors and related heterostructures
Grant ID : 682843
Förderprogramm : Horizon 2020 (H2020)
Förderorganisation : European Commission (EC)

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Titel: Physical Review Letters
  Kurztitel : Phys. Rev. Lett.
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: Woodbury, N.Y. : American Physical Society
Seiten: 6 Band / Heft: 125 (21) Artikelnummer: 216404 Start- / Endseite: - Identifikator: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1