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  Covalent triazine framework/carbon nanotube hybrids enabling selective reduction of CO2 to CO at low overpotential

Laemont, A., Abednatanzi, S., Derakshandeh, P. G., Verbruggen, F., Fiset, E., Qin, Q., et al. (2020). Covalent triazine framework/carbon nanotube hybrids enabling selective reduction of CO2 to CO at low overpotential. Green Chemistry, 22(10), 3095-3103. doi:10.1039/D0GC00090F.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0006-968B-4 Version Permalink: https://hdl.handle.net/21.11116/0000-0006-968C-3
Genre: Journal Article

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 Creators:
Laemont, Andreas, Author
Abednatanzi, Sara, Author
Derakshandeh, Parviz Gohari, Author
Verbruggen, Florian, Author
Fiset, Erika, Author
Qin, Qing1, Author           
Van Daele, Kevin, Author
Meledina, Maria, Author
Schmidt, Johannes, Author
Oschatz, Martin1, Author           
Van Der Voort, Pascal, Author
Rabaey, Korneel, Author
Antonietti, Markus2, Author           
Breugelmans, Tom, Author
Leus, Karen, Author
Affiliations:
1Martin Oschatz, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2364733              
2Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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 Abstract: Electrochemical reduction of CO2 provides a way to generate base chemicals from an abundant C1-source under mild conditions, whilst at the same time mitigating CO2 emissions. In this work, a novel class of tailorable, porous electrocatalysts for this process is proposed. Covalent triazine frameworks (CTFs) are grown in situ onto functionalized multiwalled carbon nanotubes. Hydroxyl groups decorating the surface of the multiwalled carbon nanotubes facilitate intimate contact between the carbon nanotubes and CTF, thus promoting efficient electron transfer. The novel hybrid materials generate CO with a faradaic efficiency up to 81 at an overpotential of 380 mV. The selectivity of the electrocatalysts could be linked to the amount of nitrogen present within the framework.

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Language(s): eng - English
 Dates: 2020-02-132020
 Publication Status: Issued
 Pages: -
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 Table of Contents: -
 Rev. Type: -
 Identifiers: DOI: 10.1039/D0GC00090F
BibTex Citekey: D0GC00090F
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Title: Green Chemistry
  Other : Green Chem.
Source Genre: Journal
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Publ. Info: Cambridge, UK : Royal Society of Chemistry
Pages: - Volume / Issue: 22 (10) Sequence Number: - Start / End Page: 3095 - 3103 Identifier: ISSN: 1463-9262