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  Photoactive graphitic carbon nitride-based gel beads as recyclable photocatalysts

Cao, Q., Barrio, J., Antonietti, M., Kumru, B., Shalom, M., & Schmidt, B. V. K. J. (2020). Photoactive graphitic carbon nitride-based gel beads as recyclable photocatalysts. ACS applied polymer materials. doi:10.1021/acsapm.0c00453.

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Item Permalink: http://hdl.handle.net/21.11116/0000-0006-AA00-A Version Permalink: http://hdl.handle.net/21.11116/0000-0006-AA01-9
Genre: Journal Article

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 Creators:
Cao, Qian1, Author              
Barrio, Jesus, Author
Antonietti, Markus2, Author              
Kumru, Baris3, Author              
Shalom, Menny, Author
Schmidt, Bernhard V. K. J.1, Author              
Affiliations:
1Bernhard Schmidt, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2149676              
2Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              
3Baris Kumru, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_3202957              

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Free keywords: hydrogel beads; photocatalysis; waste water remediation; carbon nitride; suspension polymerization; photopolymerization
 Abstract: Photocatalysis for clean hydrogen production and waste water remediation holds a great promise on society. However, despite the significant progress in this field the recyclability of the photocatalytic materials together with good photoactivity remain a great challenge. photocatalytic materials for waste water cleaning and hydrogen production based on the utilization of photoactive macrogel beads as the photocatalyst. To do so, we design a graphitic carbon nitride based macrogels with tailored size, swelling behavior and photocatalytic properties. Detailed studies reveal that the catalytic activity is correlated with the polymer particle size, g-C3N4 content and swelling behavior, enabling the optimization of the photocatalytic processes. We believe that the presented strategy together with the good photocatalytic activity and excellent recyclability constitute open the path for a substantial progress in this field.

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Language(s): eng - English
 Dates: 2020-06-292020
 Publication Status: Published in print
 Pages: -
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 Table of Contents: -
 Rev. Method: -
 Identifiers: DOI: 10.1021/acsapm.0c00453
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Title: ACS applied polymer materials
  Other : ACS appl. polym. mater.
Source Genre: Journal
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Publ. Info: Washington, DC : American Chemical Society
Pages: - Volume / Issue: - Sequence Number: - Start / End Page: - Identifier: ISSN: 2637-6105