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  The second-harmonic response of single-crystal silver electrodes obtained with an interference method

Beltramo, G. L., Bilger, C., Pettinger, B., & Schmickler, W. (1998). The second-harmonic response of single-crystal silver electrodes obtained with an interference method. Chemical Physics, 238(3), 473-480. doi:10.1016/S0301-0104(98)00343-7.

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 Creators:
Beltramo, Guillermo L.1, Author
Bilger, Christoph2, Author              
Pettinger, Bruno2, Author              
Schmickler, Wolfgang1, Author
Affiliations:
1Abteilung Elektrochemie, University of Ulm, ou_persistent22              
2Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              

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 Abstract: The second-harmonic response of several single-crystal silver electrodes is investigated at a long wavelength. In contrast to earlier experiments, the phase of the signal is obtained directly by an interference method. By comparing measurements at two different angles of incidence, the Rudnick-Stern coefficient characterizing the response perpendicular to the surface can be estimated; for Ag(100) and Ag(111) it agrees fairly well with calculations based on the jellium model. For the Ag(110) surface, the twofold amplitude depends on the electrode potential; in addition, a contribution with a three-fold symmetry is observed. These unexpected features are probably caused by a facetting of the Ag(110) surface. (C) 1998 Elsevier Science B.V. All rights reserved.

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Language(s): eng - English
 Dates: 1998-05-151998-06-181998-12-01
 Publication Status: Published in print
 Pages: 8
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1016/S0301-0104(98)00343-7
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Title: Chemical Physics
  Other : Chem. Phys.
Source Genre: Journal
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Publ. Info: Amsterdam : Elsevier B.V.
Pages: 8 Volume / Issue: 238 (3) Sequence Number: - Start / End Page: 473 - 480 Identifier: ISSN: 0301-0104
CoNE: https://pure.mpg.de/cone/journals/resource/954925509371