English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT
Add to Basket
 Local TagsRelease HistoryDetailsSummary
  Vibrational coherent control of localized d–d electronic excitation

Marciniak, A., Marcantoni, S., Giusti, F., Glerean, F., Sparapassi, G., Nova, T. F., et al. (2021). Vibrational coherent control of localized d–d electronic excitation. Nature Physics, 17(3), 368-373. doi:10.1038/s41567-020-01098-8.

Item is

 

show all hide all

Basic

show hide
Item Permalink: https://hdl.handle.net/21.11116/0000-0006-D622-2 Version Permalink: https://hdl.handle.net/21.11116/0000-000B-C639-6
Genre: Journal Article

Files

show Files
hide Files
:
2003.13447.pdf (Preprint), 5MB
View   Save
File Permalink:
https://hdl.handle.net/21.11116/0000-0006-D624-0
Name:
2003.13447.pdf
Description:
Downloaded from arxiv.org: 2020-08-12
OA-Status:
Not specified
Visibility:
Public
MIME-Type / Checksum:
application/pdf / [MD5]
Technical Metadata:
View
Copyright Date:
2020
Copyright Info:
© the Author(s)
License:
https://arxiv.org/help/license
:
suppl.zip (Supplementary material), 5MB
View   Save
File Permalink:
https://hdl.handle.net/21.11116/0000-0007-A0DF-9
Name:
suppl.zip
Description:
Supplementary Figs. 1–11, experimental details, complementary results, discussion, details about the theory and calculations, and Tables 1 and 2. (pdf); Source data for Fig. 1c.(xlsx); Source data for Fig. 2 (xlsx); Source data for Fig. 3. (xlsx)
OA-Status:
Not specified
Visibility:
Public
MIME-Type / Checksum:
application/zip / [MD5]
Technical Metadata:
View
Copyright Date:
-
Copyright Info:
-
License:
-
:
s41567-020-01098-8.pdf (Publisher version), 3MB
 
File Permalink:
-
Name:
s41567-020-01098-8.pdf
Description:
-
OA-Status:
Visibility:
Private
MIME-Type / Checksum:
application/pdf
Technical Metadata:
Copyright Date:
-
Copyright Info:
-
License:
-

Locators

show
hide
Locator:
https://arxiv.org/abs/2003.13447 (Preprint)
Description:
-
OA-Status:
Not specified
Locator:
https://dx.doi.org/10.1038/s41567-020-01098-8 (Publisher version)
Description:
-
OA-Status:
Not specified

Creators

show
hide
 Creators:
Marciniak, A.1, 2, Author
Marcantoni, S.1, 3, Author
Giusti, F.1, 2, Author
Glerean, F.1, 2, Author
Sparapassi, Giorgia1, 2, Author
Nova, T. F.4, Author           
Cartella, A.4, Author           
Latini, S.5, Author           
Valiera, F.1, Author
Rubio, A.5, Author           
van den Brink, J.6, 7, Author
Benatti, F.1, 3, Author
Fausti, D.1, 2, 8, Author
Affiliations:
1Department of Physics, University of Trieste, ou_persistent22              
2Elettra-Sincrotrone Trieste S.C.p.A., ou_persistent22              
3National Institute for Nuclear Physics (INFN), Trieste Section, ou_persistent22              
4Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938293              
5Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
6Leibniz Institute for Solid State and Materials Research, ou_persistent22              
7Institut für Theoretische Physik and Würzburg-Dresden Cluster of Excellence ct.qmat, Technische Universität Dresden, ou_persistent22              
8Department of Chemistry, Princeton University, ou_persistent22              

Content

show
hide
Free keywords: -
 Abstract: Addressing the role of quantum coherence in the interplay between the different matter constituents (electrons, phonons and spin) is a critical step towards understanding transition metal oxides and design complex materials with new functionalities. Here we use coherent vibrational control of onsite d-d electronic transitions in a model edge-sharing insulating transition metal oxide (CuGeO3) to single-out the effects of vibrational coherence in electron-phonon coupling. By comparing time domain experiments based on high and low frequency ultrashort pumps with a fully quantum description of phonon assisted absorption, we could distinguish the processes associated to incoherent thermal lattice fluctuations from those driven by the coherent motion of the atoms. In particular, while thermal fluctuation of the phonon bath uniformly increases the electronic absorption, the resonant excitation of phonon modes results also in light-induced transparency which is coherently controlled by the vibrational motion.

Details

show
hide
Language(s): eng - English
 Dates: 2020-02-172020-10-122021-01-042021-03
 Publication Status: Issued
 Pages: 8
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: arXiv: 2003.13447
DOI: 10.1038/s41567-020-01098-8
 Degree: -

Event

show

Legal Case

show

Project information

show hide
Project name : We thank A. Revcolevschi for providing the CuGeO3 samples and the critical reading of the manuscript and A. Cavalleri for his feedback on the manuscript and project. This work was mainly supported by the ERC grant INCEPT no. 677488. F. Glerean was supported by the Italian Ministry of Education, University and Research, MIUR (SIR project grant no. RBSI14ZIY2). This work was partially supported by the European Research Council (ERC-2015-AdG694097), the Cluster of Excellence AIM and SFB925. J.v.d.B. aknowledges support from the Deutsche Forschungsgemeinschaft (DFG) through the Würzburg-Dresden Cluster of Excellence ct.qmat (EXC 2147, project ID 390858490) and CRC 1143 (project no. A05, project ID 247310070). F.B. acknowledges that his research has been conducted within the framework of the Trieste Institute for Theoretical Quantum Technologies.
Grant ID : -
Funding program : -
Funding organization : -

Source 1

show
hide
Title: Nature Physics
  Other : Nat. Phys.
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: London : Nature Pub. Group
Pages: - Volume / Issue: 17 (3) Sequence Number: - Start / End Page: 368 - 373 Identifier: ISSN: 1745-2473
CoNE: https://pure.mpg.de/cone/journals/resource/1000000000025850