Double Core-Hole Generation in O2 Molecules Using an X-Ray Free-Electron Laser: 
Molecular-Frame Photoelectron Angular Distributions

Kastirke, Gregor; Schöffler, Markus S.; Weller, Miriam; Rist, Jonas; Boll, Rebecca; Anders, Nils; Baumann, Thomas M.; Eckart, Sebastian; Erk, Benjamin; De Fanis, Alberto; Fehre, Killian; Gatton, Averell; Grundmann, Sven; Grychtol, Patrik; Hartung, Alexander; Hofmann, Max; Ilchen, Markus; Janke, Christian; Kircher, Max; Kunitski, Maksim; Li, Xiang; Mazza, Tommaso; Melzer, Niklas; Montano, Jacobo; Music, Valerija; Nalin, Giammarco; Ovcharenko, Yevheniy; Pier, Andreas; Rennhack, Nils; Rivas, Daniel E.; Dörner, Reinhard; Rolles, Daniel; Rudenko, Artem; Schmidt, Phillipp; Siebert, Juliane; Stenger, Nico; Trabert, Daniel; Vela-Perez, Isabel; Wagner, Rene; Weber, Thorsten; Williams, Joshua B.; Ziolkowski, Pawel; Schmidt, Lothar Ph. H.; Czasch, Achim; Ueda, Kiyoshi; Trinter, Florian; Meyer, Michael; Demekhin, Philipp V.; Jahnke, Till

doi:10.1103/PhysRevLett.125.163201

Local TagsRelease HistoryDetailsSummary

Double Core-Hole Generation in O₂ Molecules Using an X-Ray Free-Electron Laser: Molecular-Frame Photoelectron Angular Distributions

Kastirke, G., Schöffler, M. S., Weller, M., Rist, J., Boll, R., Anders, N., et al. (2020). Double Core-Hole Generation in O₂ Molecules Using an X-Ray Free-Electron Laser: Molecular-Frame Photoelectron Angular Distributions. Physical Review Letters, 125(16): 163201. doi:10.1103/PhysRevLett.125.163201.

Item is Released

show all hide all

Basic

show hide

Item Permalink: https://hdl.handle.net/21.11116/0000-0007-45DD-3 Version Permalink: https://hdl.handle.net/21.11116/0000-0009-5F4B-A

Genre: Journal Article

Files

show Files

hide Files

:

PhysRevLett.125.163201.pdf (Publisher version), 515KB

View Save

File Permalink:
https://hdl.handle.net/21.11116/0000-0007-45DF-1

Name:
PhysRevLett.125.163201.pdf

Description:
-

OA-Status:

Visibility:
Public

MIME-Type / Checksum:
application/pdf / [MD5]

Technical Metadata:

View

Copyright Date:
2020

Copyright Info:
The Author(s)

License:
https://creativecommons.org/licenses/by/4.0/

Locators

show

Creators

show

hide

Creators:
Kastirke, Gregor¹, Author
Schöffler, Markus S.¹, Author
Weller, Miriam¹, Author
Rist, Jonas¹, Author
Boll, Rebecca², Author
Anders, Nils¹, Author
Baumann, Thomas M.², Author
Eckart, Sebastian¹, Author
Erk, Benjamin³, Author
De Fanis, Alberto², Author
Fehre, Killian¹, Author
Gatton, Averell⁴, Author
Grundmann, Sven¹, Author
Grychtol, Patrik², Author
Hartung, Alexander¹, Author
Hofmann, Max¹, Author
Ilchen, Markus^{2, 5}, Author
Janke, Christian¹, Author
Kircher, Max¹, Author
Kunitski, Maksim¹, Author
Li, Xiang⁶, AuthorMazza, Tommaso², AuthorMelzer, Niklas¹, AuthorMontano, Jacobo², AuthorMusic, Valerija^{2, 5}, AuthorNalin, Giammarco¹, AuthorOvcharenko, Yevheniy², AuthorPier, Andreas¹, AuthorRennhack, Nils², AuthorRivas, Daniel E.², AuthorDörner, Reinhard¹, AuthorRolles, Daniel⁶, AuthorRudenko, Artem⁶, AuthorSchmidt, Phillipp^{2, 5}, AuthorSiebert, Juliane¹, AuthorStenger, Nico¹, AuthorTrabert, Daniel¹, AuthorVela-Perez, Isabel¹, AuthorWagner, Rene², AuthorWeber, Thorsten⁷, AuthorWilliams, Joshua B.⁸, AuthorZiolkowski, Pawel², AuthorSchmidt, Lothar Ph. H.¹, AuthorCzasch, Achim¹, AuthorUeda, Kiyoshi⁹, AuthorTrinter, Florian^{3, 10}, Author Meyer, Michael², AuthorDemekhin, Philipp V.⁵, AuthorJahnke, Till¹, Author more..

Affiliations:
1Institut für Kernphysik, Goethe-Universität, Max-von-Laue-Strasse 1, 60438 Frankfurt am Main, Germany, ou_persistent22
2European XFEL GmbH, Holzkoppel 4, 22869 Schenefeld, Germany, ou_persistent22
3Deutsches Elektronen-Synchrotron (DESY), Notkestrasse 85, 22607 Hamburg, Germany, ou_persistent22
4SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA, ou_persistent22
5Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Strasse 40, 34132 Kassel, Germany, ou_persistent22
6J.R. Macdonald Laboratory, Department of Physics, Kansas State University, Manhattan, Kansas 66506, USA, ou_persistent22
7Lawrence Berkeley National Laboratory, Chemical Sciences Division, Berkeley, California 94720, USA, ou_persistent22
8Department of Physics, University of Nevada, Reno, Nevada 89557, USA, ou_persistent22
9Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Sendai 980-8577, Japan, ou_persistent22
10Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545

Content

show

hide

Free keywords: -

Abstract: We report on a multiparticle coincidence experiment performed at the European X-ray Free-ElectronLaser at the Small Quantum Systems instrument using a COLTRIMS reaction microscope. By measuringtwo ions and two electrons in coincidence, we investigate double core-hole generation in O₂ molecules inthe gas phase. Single-site and two-site double core holes have been identified and their molecular-frameelectron angular distributions have been obtained for a breakup of the oxygen molecule into two doublycharged ions. The measured distributions are compared to results of calculations performed within thefrozen- and relaxed-core Hartree-Fock approximations.

Details

show

hide

Language(s): eng - English

Dates: Submitted: 2020-05-07Accepted: 2020-10-14Published Online: 2020-10-14Date issued: 2020-10-16

Publication Status: Issued

Pages: 6

Publishing info: -

Table of Contents: -

Rev. Type: Peer

Identifiers: DOI: 10.1103/PhysRevLett.125.163201

Degree: -

Event

show

Legal Case

show

Project information

show

Source 1

show

hide

Title: Physical Review Letters

Abbreviation : Phys. Rev. Lett.

Source Genre: Journal

Creator(s):

Affiliations:

Publ. Info: Woodbury, N.Y. : American Physical Society

Pages: 6 Volume / Issue: 125 (16) Sequence Number: 163201 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1