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  Mass Accommodation and Gas-Particle Partitioning in Secondary Organic Aerosols: Dependence on Diffusivity, Volatility, Particle-phase Reactions, and Penetration Depth

Garfinkel, C. I., Harari, O., Ziskin, S., Rao, J., Morgenstern, O., Zeng, G., et al. (2020). Mass Accommodation and Gas-Particle Partitioning in Secondary Organic Aerosols: Dependence on Diffusivity, Volatility, Particle-phase Reactions, and Penetration Depth. Atmospheric Chemistry and Physics Discussions, 20. doi:10.5194/acp-2020-801.

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 Creators:
Garfinkel, Chaim Israel, Author
Harari, Ohad, Author
Ziskin, Shlomi, Author
Rao, Jian, Author
Morgenstern, Olaf, Author
Zeng, Guang, Author
Tilmes, Simone, Author
Kinnison, Doug, Author
O'Connor, Fiona M., Author
Butchart, Neal, Author
Deushi, Makoto, Author
Jöckel, Patrick, Author
Pozzer, Andrea1, Author              
Affiliations:
1Atmospheric Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826285              

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 Abstract: The connection between the dominant mode of interannual variability in the tropical troposphere, El Nino Southern Oscillation (ENSO), and entry of stratospheric water vapor, is analyzed in a set of the model simulations archived for the Chemistry-Climate Model Initiative (CCMI) project and for phase 6 of the Coupled Model Intercomparison Project. While the models agree on the temperature response to ENSO in the tropical troposphere and lower stratosphere, and all models also agree on the zonal structure of the response in the tropical tropopause layer, the only aspect of the entry water vapor with consensus is that La Nina leads to moistening in winter relative to neutral ENSO. For El Nino and for other seasons there are significant differences among the models. For example, some models find that the enhanced water vapor for La Nina in the winter of the event reverses in spring and summer, other models find that this moistening persists, while some show a nonlinear response with both El Nino and La Nina leading to enhanced water vapor in both winter, spring, and summer. Focusing on Central Pacific ENSO versus East Pacific ENSO, or temperatures in the mid-troposphere as compared to temperatures near the surface, does not narrow the inter-model discrepancies. Despite this diversity in response, the temperature response near the cold point can explain the response of water vapor when each model is considered separately. While the observational record is too short to fully constrain the response to ENSO, it is clear that most models suffer from biases in the magnitude of interannual variability of entry water vapor. This bias could be due to missing forcing processes that contribute to observed variability in cold point temperatures.

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Language(s): eng - English
 Dates: 2020-09-10
 Publication Status: Published online
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: No review
 Identifiers: DOI: 10.5194/acp-2020-801
 Degree: -

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Title: Atmospheric Chemistry and Physics Discussions
  Abbreviation : Atmos. Chem. Phys. Discuss.
Source Genre: Journal
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Publ. Info: Katlenburg-Lindau, Germany : European Geophysical Society, Copernicus Publ.
Pages: 23 Volume / Issue: 20 Sequence Number: - Start / End Page: - Identifier: ISSN: 1680-7367
CoNE: https://pure.mpg.de/cone/journals/resource/111076360006006