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  Flexibilization of Biorefineries: Tuning Lignin Hydrogenation by Hydrogen Partial Pressure

Cao, Z., Xu, Y., Lyu, P., Dierks, M., Morales‐García, Á., Schrader, W., et al. (2021). Flexibilization of Biorefineries: Tuning Lignin Hydrogenation by Hydrogen Partial Pressure. ChemSusChem, 14(1), 373-378. doi:10.1002/cssc.202002248.

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Genre: Journal Article

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 Creators:
Cao, Zhengwen1, Author           
Xu, Yun2, Author           
Lyu, Pengbo3, Author
Dierks, Michael1, Author           
Morales‐García, Ángel3, Author
Schrader, Wolfgang2, Author           
Nachtigall, Petr3, Author
Schüth, Ferdi1, Author           
Affiliations:
1Research Department Schüth, Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445589              
2Service Department Schrader (MS), Max-Planck-Institut für Kohlenforschung, Max Planck Society, ou_1445629              
3Department of Physical and Macromolecular Chemistry, Faculty of Science, Charles University, 128 43 Prague 2, Czech Republic, ou_persistent22              

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Free keywords: biomass; hydrogen; lignin; renewable energy; waste valorization
 Abstract: The present study describes an interesting and practical catalytic system that allows flexible conversion of lignin into aromatic or aliphatic hydrocarbons, depending on the hydrogen partial pressure. A combination of experiment and theory shows that the product distribution between aromatics and aliphatics can be simply tuned by controlling the availability of hydrogen on the catalyst surface. Noticeably, these pathways lead to almost complete oxygen removal from lignin biomass, yielding high‐quality hydrocarbons. Thus, hydrogen–lignin co‐refining by using this catalytic system provides high flexibility in hydrogen storage/consumption towards meeting different regional and temporal demands.

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Language(s): eng - English
 Dates: 2020-09-222020-11-112021-01-07
 Publication Status: Published online
 Pages: 6
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1002/cssc.202002248
 Degree: -

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Title: ChemSusChem
Source Genre: Journal
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Publ. Info: Weinheim : Wiley-VCH
Pages: - Volume / Issue: 14 (1) Sequence Number: - Start / End Page: 373 - 378 Identifier: ISSN: 1864-5631
CoNE: https://pure.mpg.de/cone/journals/resource/1864-5631