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  Laser-carbonization : peering into the formation of micro-thermally produced (N-doped)carbons

Wang, H., Delacroix, S., Osswald, O., Anderson, M., Heil, T., Lepre, E., et al. (2021). Laser-carbonization: peering into the formation of micro-thermally produced (N-doped)carbons. Carbon, 176, 500-510. doi:10.1016/j.carbon.2021.01.145.

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 Creators:
Wang, Huize1, Author           
Delacroix, Simon1, Author           
Osswald, Oliver, Author
Anderson, Mackenzie, Author
Heil, Tobias2, Author           
Lepre, Enrico3, Author                 
Lopez Salas, Nieves3, Author                 
Kaner, Richard B., Author
Smarsly, Bernd, Author
Strauß, Volker4, Author           
Affiliations:
1Volker Strauß, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_3025555              
2Nadezda V. Tarakina, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2522693              
3Nieves Lopez Salas, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_3029702              
4Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863288              

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Free keywords: Carbonization, Laser-carbonization, N-doped carbon, Carbon laser patterning, WAXS, Wide-angle X-ray scattering
 Abstract: Even after centuries-old experience in carbonizing materials we can still learn new lessons and find new applications for carbonized materials. In the past decades, laser-assisted syntheses of materials have emerged as versatile tools for the fabrication of micro- and nanostructured functional devices. In this regard, laser-carbonization is of particular interest, as it provides a method for patterning eco-friendly and potentially biodegradable electronic materials for future applications in comparison to the state-of-the-art in flexible electronics. However, using molecular precursors for laser-carbonization has been a challenge for many years. We identified a set of three different precursors and conducted an in-depth morphological and compositional study to understand how molecular precursors must be prepared for the high-speed carbonization reactions used in laser-patterning. The resulting laser-patterned carbons (LP-C) or N-doped carbons (LP-NC) are different from their conventionally pyrolyzed reference products mostly in terms of morphology. A generally porous structure and a carbonization gradient induced by the top-to-bottom energy input are the most remarkable features. Additionally, the microstructure, the elemental composition and the resulting electronic properties are different as demonstrated by X-ray photoelectron spectroscopy (XPS) and wide-angle X-ray scattering (WAXS) analysis.

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Language(s): eng - English
 Dates: 2021-01-312021
 Publication Status: Issued
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: -
 Identifiers: DOI: 10.1016/j.carbon.2021.01.145
BibTex Citekey: WANG2021500
 Degree: -

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Title: Carbon
  Abbreviation : Carbon
Source Genre: Journal
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Publ. Info: Amsterdam : Elsevier
Pages: - Volume / Issue: 176 Sequence Number: - Start / End Page: 500 - 510 Identifier: ISSN: 0008-6223