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  Physisorption of CO and N2 on Al(111): Observation of surface-molecule vibrations in electron resonance scattering

Jacobi, K., & Bertolo, M. (1990). Physisorption of CO and N2 on Al(111): Observation of surface-molecule vibrations in electron resonance scattering. Physical Review B, 42(6), 3733-3736. doi:10.1103/PhysRevB.42.3733.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0008-3CBA-4 Version Permalink: https://hdl.handle.net/21.11116/0000-0008-3FE9-C
Genre: Journal Article

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 Creators:
Jacobi, Karl1, Author           
Bertolo, M.2, Author           
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
2Fritz Haber Institute, Max Planck Society, ou_24021              

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 Abstract: Monolayers of physisorbed CO and N2 on Al(111) were investigated by means of high-resolution electron-energy-loss spectroscopy (HREELS). The line shapes of the ν=0→1 molecular stretching modes differ largely. In the high-energy-loss tail of this mode, surface-molecule stretching losses are detected with an energy of 10.5 meV in the case of N2. It is demonstrated that this large inelastic intensity is due to the negative-ion resonance scattering mode operating for N2 but not for CO. The results are discussed in the framework of Gadzuk’s wave-packet method for time-dependent quantum behavior of molecules on surfaces.

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Language(s): eng - English
 Dates: 1990-04-241990-08-15
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevB.42.3733
 Degree: -

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Title: Physical Review B
  Abbreviation : Phys. Rev. B
Source Genre: Journal
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Publ. Info: Woodbury, NY : American Physical Society
Pages: 4 Volume / Issue: 42 (6) Sequence Number: - Start / End Page: 3733 - 3736 Identifier: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008