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  Detection of photon statistics and multimode field correlations by Raman processes

Schlawin, F., Dorfman, K. E., & Mukamel, S. (2021). Detection of photon statistics and multimode field correlations by Raman processes. The Journal of Chemical Physics, 154(10): 104116. doi:10.1063/5.0039759.

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 Creators:
Schlawin, F.1, 2, Author           
Dorfman, K. E.3, Author
Mukamel, S.4, Author
Affiliations:
1The Hamburg Centre for Ultrafast Imaging, ou_persistent22              
2Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938285              
3State Key Laboratory of Precision Spectroscopy, East China Normal University, ou_persistent22              
4Department of Chemistry and Physics & Astronomy, University of California, ou_persistent22              

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 Abstract: Glauber’s g^(2)-function provides a common measure of quantum field statistics through two-photon coincidence counting in Hanbury Brown–Twiss measurements. Here, we propose to use nonlinear optical signals as a tool for the characterization of quantum light. In particular, we show that Raman measurements provide an alternative direct probe for a different component of the four-point correlation function underlying the g^(2)-function. We illustrate this capacity for a specific quantum state obtained from a frequency conversion process. Our work points out how the analysis of controlled optical nonlinear processes can provide an alternative window toward the analysis of quantum light sources.

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Language(s): eng - English
 Dates: 2020-12-062021-02-162021-03-102021-03-14
 Publication Status: Issued
 Pages: -
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 Rev. Type: Peer
 Identifiers: DOI: 10.1063/5.0039759
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Project name : F.S. acknowledges support from the Cluster of Excellence “Advanced Imaging of Matter” of the Deutsche Forschungsgemeinschaft (DFG)—EXC 2056—Project No. 390715994. K.E.D. gratefully acknowledges the support from the National Science Foundation of China (Grant No. 11934011), the Zijiang Endowed Young Scholar Fund, East China Normal University, and the Overseas Expertise Introduction Project for Discipline Innovation (Grant Nos. 111 Project and B12024). S.M. gratefully acknowledges the support of the National Science Foundation through Grant No. CHE-1953045 and the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-FG02-04ER1557 which also supported visits by K.E.D. to the University of California, Irvine.
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Title: The Journal of Chemical Physics
  Abbreviation : J. Chem. Phys.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Institute of Physics
Pages: - Volume / Issue: 154 (10) Sequence Number: 104116 Start / End Page: - Identifier: ISSN: 0021-9606
CoNE: https://pure.mpg.de/cone/journals/resource/954922836226