Deutsch
 
Hilfe Datenschutzhinweis Impressum
  DetailsucheBrowse

Datensatz

DATENSATZ AKTIONENEXPORT
Zur Ablage hinzufügen
 Lokale TagsFreigabegeschichteDetailsÜbersicht
  Potential energy-driven spin manipulation via a controllable hydrogen ligand

Jacobson, P., Muenks, M., Laskin, G., Brovko, O., Stepanyuk, V., Ternes, M., et al. (2017). Potential energy-driven spin manipulation via a controllable hydrogen ligand. Science Advances, 3(4): e1602060. doi:10.1126/sciadv.1602060.

Item is

 

einblenden: alle ausblenden: alle

Basisdaten

einblenden: ausblenden:
Datensatz-Permalink: https://hdl.handle.net/21.11116/0000-000B-24ED-2 Versions-Permalink: https://hdl.handle.net/21.11116/0000-000B-24EE-1
Genre: Zeitschriftenartikel

Dateien

einblenden: Dateien
ausblenden: Dateien
:
sciadv.1602060.pdf (Verlagsversion), 681KB
Öffnen   Speichern
Datei-Permalink:
https://hdl.handle.net/21.11116/0000-000B-24EF-0
Name:
sciadv.1602060.pdf
Beschreibung:
-
OA-Status:
Gold
Sichtbarkeit:
Öffentlich
MIME-Typ / Prüfsumme:
application/pdf / [MD5]
Technische Metadaten:
Öffnen
Copyright Datum:
2017
Copyright Info:
The Author(s)
Lizenz:
http://creativecommons.org/licenses/by-nc/4.0/

Externe Referenzen

einblenden:
ausblenden:
externe Referenz:
https://doi.org/10.1126/sciadv.1602060 (Verlagsversion)
Beschreibung:
-
OA-Status:
Gold

Urheber

einblenden:
ausblenden:
 Urheber:
Jacobson, Peter1, Autor
Muenks, Matthias1, Autor
Laskin, Gennadii1, Autor
Brovko, Oleg1, Autor
Stepanyuk, Valeri2, Autor
Ternes, Markus1, Autor
Kern, Klaus1, Autor
Affiliations:
1External Organizations, ou_persistent22              
2Max Planck Institute of Microstructure Physics, Max Planck Society, Weinberg 2, 06120 Halle, DE, ou_2415691              

Inhalt

einblenden:
ausblenden:
Schlagwörter: -
 Zusammenfassung: Spin-bearing molecules can be stabilized on surfaces and in junctions with desirable properties, such as a net spin that can be adjusted by external stimuli. Using scanning probes, initial and final spin states can be deduced from topographic or spectroscopic data, but how the system transitions between these states is largely unknown. We address this question by manipulating the total spin of magnetic cobalt hydride complexes on a corrugated boron nitride surface with a hydrogen-functionalized scanning probe tip by simultaneously tracking force and conductance. When the additional hydrogen ligand is brought close to the cobalt monohydride, switching between a correlated S = 1/2 Kondo state, where host electrons screen the magnetic moment, and an S = 1 state with magnetocrystalline anisotropy is observed. We show that the total spin changes when the system is transferred onto a new potential energy surface that is defined by the position of the hydrogen in the junction. These results show how and why chemically functionalized tips are an effective tool to manipulate adatoms and molecules and a promising new method to selectively tune spin systems.

Details

einblenden:
ausblenden:
Sprache(n):
 Datum: 2017-04-142017-04-07
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: -
 Identifikatoren: BibTex Citekey: P12936
DOI: 10.1126/sciadv.1602060
 Art des Abschluß: -

Veranstaltung

einblenden:

Entscheidung

einblenden:

Projektinformation

einblenden:

Quelle 1

einblenden:
ausblenden:
Titel: Science Advances
  Andere : Sci. Adv.
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: Washington : AAAS
Seiten: - Band / Heft: 3 (4) Artikelnummer: e1602060 Start- / Endseite: - Identifikator: ISSN: 2375-2548
CoNE: https://pure.mpg.de/cone/journals/resource/2375-2548