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  Antiferromagnetism and phase transitions in noncentrosymmetric UIrSi3

Valenta, J., Honda, F., Vališka, M., Opletal, P., Kaštil, J., Míšek, M., et al. (2018). Antiferromagnetism and phase transitions in noncentrosymmetric UIrSi3. Physical Review B, 97(14): 144423. doi:10.1103/PhysRevB.97.144423.

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 Creators:
Valenta, J.1, Author
Honda, F.1, Author
Vališka, M.1, Author
Opletal, P.1, Author
Kaštil, J.1, Author
Míšek, M.1, Author
Diviš, M.1, Author
Sandratskii, L. M.2, Author
Prchal, J.1, Author
Sechovsky, V.1, Author
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1External Organizations, ou_persistent22              
2Max Planck Institute of Microstructure Physics, Max Planck Society, Weinberg 2, 06120 Halle, DE, ou_2415691              

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 Abstract: Magnetization and specific-heat measurements on a UIrSi3 single crystal reveal Ising-like antiferromagnetism below TN=41.7K with the easy magnetization direction along the c axis of the tetragonal structure. The antiferromagnetic ordering is suppressed by magnetic fields >Hc0Hc=7.3T at 2 K) applied along the c axis. The first-order metamagnetic transition at Hc exhibits asymmetric hysteresis reflecting a slow reentry of the complex ground-state antiferromagnetic structure with decreasing field. The hysteresis narrows with increasing temperature and vanishes at 28 K. A second-order metamagnetic transition is observed at higher temperatures. The point of change of the order of transition in the established H-T magnetic phase diagram is considered as the tricritical point (at Ttc=28K and μ0Htc=5.8T). The modified-Curie-Weiss law fits of temperature dependence of the a- and c-axis susceptibility provide opposite signs of Weiss temperatures, Θpa∼−51K and Θpc∼+38K, respectively. This result and the small value of μ0Hc contrasting to the high TN indicate competing ferromagnetic and antiferromagnetic interactions responsible for the complex antiferromagnetic ground state. The simultaneous electronic-structure calculations focused on the total energy of ferromagnetic and various antiferromagnetic states, the U magnetic moment, and magnetocrystalline anisotropy provide results consistent with experimental findings and the suggested physical picture of the system.

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 Dates: 2018-04-302018-04-01
 Publication Status: Issued
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 Identifiers: BibTex Citekey: P13243
DOI: 10.1103/PhysRevB.97.144423
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Title: Physical Review B
  Abbreviation : Phys. Rev. B
Source Genre: Journal
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Publ. Info: Woodbury, NY : American Physical Society
Pages: - Volume / Issue: 97 (14) Sequence Number: 144423 Start / End Page: - Identifier: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008