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  Spin density localization and accessibility in organic radicals for liquid-state DNP efficiency

Levien, M., Reinhard, M., Hiller, M., Tkach, I., Bennati, M., & Orlando, T. (2021). Spin density localization and accessibility in organic radicals for liquid-state DNP efficiency. Physical Chemistry Chemical Physics, 23(8), 4480-4485. doi:10.1039/D0CP05796G.

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 Creators:
Levien, M.1, Author              
Reinhard, M.2, Author              
Hiller, M.2, Author              
Tkach, I.3, Author              
Bennati, Marina2, Author              
Orlando, T.2, Author              
Affiliations:
1Research Group of Electron Paramagnetic Resonance, Max Planck Institute for Biophysical Chemistry, Max Planck Society, ou_578606              
2Research Group of Electron Paramagnetic Resonance, MPI for Biophysical Chemistry, Max Planck Society, ou_578606              
3Research Group of Electron Paramagnetic Resonance, MPI for biophysical chemistry, Max Planck Society, ou_578606              

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 Abstract: We report a large variation in liquid DNP performance of up to a factor of about five in coupling factor among organic radicals commonly used as polarizing agents. A comparative study of 1H and 13C DNP in model systems shows the impact of the spin density distribution and accessibility of the radical site by the target molecule.

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Language(s): eng - English
 Dates: 2021-02-052021-02-28
 Publication Status: Published in print
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 Rev. Type: Peer
 Identifiers: DOI: 10.1039/D0CP05796G
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Title: Physical Chemistry Chemical Physics
Source Genre: Journal
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Pages: - Volume / Issue: 23 (8) Sequence Number: - Start / End Page: 4480 - 4485 Identifier: -