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  Table-top extreme ultraviolet second harmonic generation

Helk, T., Berger, E., Jammuch, S., Hoffmann, L., Kabacinski, A., Gautier, J., et al. (2021). Table-top extreme ultraviolet second harmonic generation. Science Advances, 7(21): eabe2265. doi:10.1126/sciadv.abe2265.

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eabe2265.full.pdf (Verlagsversion), 507KB
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2021
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Helk, Tobias1, 2, Autor
Berger, Emma3, 4, Autor
Jammuch, Sasawat5, Autor
Hoffmann, Lars6, Autor           
Kabacinski, Adeline7, Autor
Gautier, Julien7, Autor
Tissandier, Fabien7, Autor
Goddet, Jean-Phillipe7, Autor
Chang, Hung-Tzu3, Autor
Oh, Juwon3, Autor
Pemmaraju, C. Das8, Autor
Pascal, Tod A.5, 9, 10, Autor
Sebban, Stephane7, Autor
Spielmann, Christian1, 2, Autor
Zürch, Michael1, 3, 4, 6, Autor           
Affiliations:
1Institute of Optics and Quantum Electronics, Abbe Center of Photonics, Friedrich-Schiller University, 07743 Jena, Germany., ou_persistent22              
2Helmholtz Institute Jena, 07743 Jena, Germany., ou_persistent22              
3Department of Chemistry, University of California, Berkeley, Berkeley, CA 94720, USA, ou_persistent22              
4Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA., ou_persistent22              
5ATLAS Materials Physics Laboratory, Department of NanoEngineering and Chemical Engineering, University of California, San Diego, La Jolla, CA 92023, USA., ou_persistent22              
6Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
7Laboratoire d’Optique Appliquée, ENSTA Paris, Ecole Polytechnique, CNRS, Institut Polytechnique de Paris, Palaiseau, France, ou_persistent22              
8Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Stanford, CA 94025, USA., ou_persistent22              
9Materials Science and Engineering, University of California, San Diego, La Jolla, CA 92023, USA., ou_persistent22              
10Sustainable Power and Energy Center, University of California, San Diego, La Jolla, CA 92023, USA., ou_persistent22              

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 Zusammenfassung: The lack of available table-top extreme ultraviolet (XUV) sources with high enough fluxes and coherence properties has limited the availability of nonlinear XUV and x-ray spectroscopies to free-electron lasers (FELs). Here, we demonstrate second harmonic generation (SHG) on a table-top XUV source by observing SHG near the Ti M2,3 edge with a high-harmonic seeded soft x-ray laser. Furthermore, this experiment represents the first SHG experiment in the XUV. First-principles electronic structure calculations suggest the surface specificity and separate the observed signal into its resonant and nonresonant contributions. The realization of XUV-SHG on a table-top source opens up more accessible opportunities for the study of element-specific dynamics in multicomponent systems where surface, interfacial, and bulk-phase asymmetries play a driving role.

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Sprache(n): eng - English
 Datum: 2020-09-022021-03-302021-05-19
 Publikationsstatus: Online veröffentlicht
 Seiten: 6
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1126/sciadv.abe2265
 Art des Abschluß: -

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Titel: Science Advances
  Andere : Sci. Adv.
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: Washington : AAAS
Seiten: 6 Band / Heft: 7 (21) Artikelnummer: eabe2265 Start- / Endseite: - Identifikator: ISSN: 2375-2548
CoNE: https://pure.mpg.de/cone/journals/resource/2375-2548