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  Decoherence-Induced Universality in Simple Metal Cluster Photoelectron Angular Distributions

Piechaczek, A., Bartels, C., Hock, C., Rost, J. M., & von Issendorff, B. (2021). Decoherence-Induced Universality in Simple Metal Cluster Photoelectron Angular Distributions. Physical Review Letters, 126(23): 233201. doi:10.1103/PhysRevLett.126.233201.

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 Creators:
Piechaczek, Adam1, Author
Bartels, Christof1, Author
Hock, Christian1, Author
Rost, Jan M.2, Author           
von Issendorff, Bernd1, Author
Affiliations:
1external, ou_persistent22              
2Max Planck Institute for the Physics of Complex Systems, Max Planck Society, ou_2117288              

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 MPIPKS: Dynamics on nanoscale systems
 Abstract: Measured angular distributions of photoelectrons from size-selected copper and sodium cluster anions are demonstrated to exhibit a universal behavior independent of the initial electron state, cluster size, or material, which can be traced back to momentum conservation upon photoemission. Quantum simulations reproduce the universality under the assumption that multielectron dynamics localizes the emission on the cluster surface and renders the cluster opaque to photoelectrons, thereby quenching interference effects that would otherwise obscure this almost classical behavior.

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 Dates: 2021-06-112021-06-11
 Publication Status: Issued
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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 126 (23) Sequence Number: 233201 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1