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  Femtosecond Surface Vibrational Spectroscopy of CO Adsorbed on Ru(001) during Desorption

Bonn, M., Hess, C., Funk, S., Miners, J. H., Persson, B. J. N., Wolf, M., et al. (2000). Femtosecond Surface Vibrational Spectroscopy of CO Adsorbed on Ru(001) during Desorption. Physical Review Letters, 84(20), 4653-4656. doi:10.1103/PhysRevLett.84.4653.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0009-287A-2 Version Permalink: https://hdl.handle.net/21.11116/0000-0009-287D-F
Genre: Journal Article

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PhysRevLett.84.4653.pdf (Publisher version), 158KB
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2000
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APS
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 Creators:
Bonn, Mischa1, 2, Author           
Hess, Christian3, Author           
Funk, Stephan1, Author           
Miners, James H.4, Author           
Persson, Bo J. N.5, Author
Wolf, Martin1, Author           
Ertl, Gerhard1, Author           
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
2Leiden Institute of Chemistry, P.O. Box 9502, 2300 RA Leiden, The Netherlands, ou_persistent22              
3Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              
4Fritz Haber Institute, Max Planck Society, ou_24021              
5IFF, Forschungszentrum Jülich, D-52425 Jülich, Germany, ou_persistent22              

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 Abstract: Using time-resolved sum-frequency generation spectroscopy, the C-O stretch vibration of carbon monoxide adsorbed on a single-crystal Ru(001) surface is investigated during femtosecond near-IR laser excitation leading to desorption. A large transient redshift, a broadening of the resonance, and a strong decrease in intensity are observed. These originate from coupling of the C-O stretch to low-frequency modes, especially the frustrated rotation, that are highly excited in the desorption process.

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Language(s): eng - English
 Dates: 1999-12-092000-05-15
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.84.4653
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: 4 Volume / Issue: 84 (20) Sequence Number: - Start / End Page: 4653 - 4656 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1