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  Direct Observation of Vibrational Energy Delocalization on Surfaces: CO on Ru(001)

Hess, C., Wolf, M., & Bonn, M. (2000). Direct Observation of Vibrational Energy Delocalization on Surfaces: CO on Ru(001). Physical Review Letters, 85(20), 4341-4344. doi:10.1103/PhysRevLett.85.4341.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0009-473F-2 Version Permalink: https://hdl.handle.net/21.11116/0000-0009-528E-B
Genre: Journal Article

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PhysRevLett.85.4341.pdf (Publisher version), 240KB
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2000
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 Creators:
Hess, Christian1, Author           
Wolf, Martin1, Author           
Bonn, Mischa2, Author
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              
2Leiden Institute of Chemistry, P.O. Box 9502, 2300 RA Leiden, The Netherlands, ou_persistent22              

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 Abstract: We report the experimental observation of the gradual transition from a local oscillator to a two-dimensional delocalized phonon, observed for the CO-stretch vibration of carbon monoxide adsorbed on a Ru(001) surface by means of broadband-infrared saturation sum-frequency spectroscopy. The data are theoretically reproduced by an exchange model with residence times of the excitation down to 2.5 ps.

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Language(s): eng - English
 Dates: 2000-05-132000-11-13
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.85.4341
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: 4 Volume / Issue: 85 (20) Sequence Number: - Start / End Page: 4341 - 4344 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1