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  Nature and impact of charge transfer to ground-state dications in atomic and molecular environments

Küstner-Wetekam, C., Hu, X. Q., Marder, L., Schmidt, P., Ozga, C., Zindel, C., et al. (2021). Nature and impact of charge transfer to ground-state dications in atomic and molecular environments. Physical Review A, 104(4): 042802. doi:10.1103/PhysRevA.104.042802.

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PhysRevA.104.042802.pdf (Publisher version), 593KB
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PhysRevA.104.042802.pdf
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 Creators:
Küstner-Wetekam, C.1, Author
Hu, X. Q.2, Author
Marder, L.1, Author
Schmidt, Ph.3, Author
Ozga, C.1, Author
Zindel, Ch.1, Author
Otto, H.1, Author
Peng, Y. G.2, Author
Wang, J. G.2, Author
Richter, Clemens4, 5, Author           
Sisourat, N.6, Author
Hergenhahn, Uwe4, 5, Author           
Knie, A.1, Author
Ehresmann, A.1, Author
Wu, Y.2, 7, Author
Hans, A.1, Author
Affiliations:
1Institut für Physik und CINSaT, Universität Kassel, Heinrich-Plett-Straße 40, D-34132 Kassel, Germany, ou_persistent22              
2The Key Laboratory of Computational Physics, Institute of Applied Physics and Computational Mathematics, Beijing 100088, China, ou_persistent22              
3European XFEL GmbH, D-22869 Schenefeld, Germany, ou_persistent22              
4Leibniz-Institut für Oberflächenmodifizierung (IOM), Permoserstraße 15, D-04318 Leipzig, Germany, ou_persistent22              
5Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              
6Laboratoire de Chimie Physique Matière et Rayonnement, UMR 7614, Sorbonne Université, CNRS, F-75005 Paris, France, ou_persistent22              
7Center for Applied Physics and Technology, HEDPS, Peking University, Beijing 100871, China, ou_persistent22              

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 Abstract: Charge transfer processes between weakly bound entities play an important role in various chemical and biological environments. In this combined experimental and theoretical work, we investigate the nature of charge-transfer processes in homogeneous atomic and heterogeneous atomic-molecular clusters. Our results reveal fundamentally different processes to be at play in pure argon clusters compared to mixed argon-nitrogen systems: We demonstrate that the former species decay via photon-mediated charge transfer while a nonradiative direct process is found dominant in the atomic-molecular cases. Our results are of general interest for studies on charge redistribution in more complex and biologically relevant samples where molecules are involved.

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Language(s): eng - English
 Dates: 2021-03-192021-09-212021-10-062021-10
 Publication Status: Published in print
 Pages: 5
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevA.104.042802
 Degree: -

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Title: Physical Review A
  Other : Phys. Rev. A
Source Genre: Journal
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Publ. Info: New York, NY : American Physical Society
Pages: 5 Volume / Issue: 104 (4) Sequence Number: 042802 Start / End Page: - Identifier: ISSN: 1050-2947
CoNE: https://pure.mpg.de/cone/journals/resource/954925225012_2