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  Giant Topological Hall Effect in the Noncollinear Phase of Two-Dimensional Antiferromagnetic Topological Insulator MnBi4Te7

Roychowdhury, S., Singh, S., Guin, S. N., Kumar, N., Chakraborty, T., Schnelle, W., et al. (2021). Giant Topological Hall Effect in the Noncollinear Phase of Two-Dimensional Antiferromagnetic Topological Insulator MnBi4Te7. Chemistry of Materials, 33(21), 8343-8350. doi:10.1021/acs.chemmater.1c02625.

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 Creators:
Roychowdhury, Subhajit1, Author           
Singh, Sukriti1, Author           
Guin, Satya N.1, Author           
Kumar, Nitesh1, Author           
Chakraborty, Tirthankar1, Author           
Schnelle, Walter2, Author           
Borrmann, Horst3, Author           
Shekhar, Chandra4, Author           
Felser, Claudia5, Author           
Affiliations:
1Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863425              
2Walter Schnelle, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863441              
3Horst Borrmann, Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863410              
4Chandra Shekhar, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863428              
5Claudia Felser, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863429              

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 Abstract: Magnetic topological insulators provide an important platform for realizing several exotic quantum phenomena, such as the axion insulating state and the quantum anomalous Hall effect, owing to the interplay between topology and magnetism. MnBi4Te7 is a two-dimensional Z(2) antiferromagnetic (AFM) topological insulator with a Ne ' el temperature of similar to 13 K. In AFM materials, the topological Hall effect (THE) is observed owing to the existence of nontrivial spin structures. A material with noncollinearity that develops in the AFM phase rather than at the onset of the AFM order is particularly important. In this study, we observed that such an unanticipated THE starts to develop in a MnBi4Te7 single crystal when the magnetic field is rotated away from the easy axis (c-axis) of the system. Furthermore, the THE resistivity reaches a giant value of similar to 7 mu Omega-cm at 2 K when the angle between the magnetic field and the c-axis is 75 degrees. This value is significantly higher than the values for previously reported systems with noncoplanar structures. The THE can be ascribed to the noncoplanar spin structure resulting from the canted state during the spinflip transition in the ground AFM state of MnBi4Te7. The large THE at a relatively low applied field makes the MnBi4Te7 system a potential candidate for spintronic applications.

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Language(s): eng - English
 Dates: 2021-10-192021-10-19
 Publication Status: Issued
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Title: Chemistry of Materials
  Abbreviation : Chem. Mater.
Source Genre: Journal
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Publ. Info: Washington, D.C. : American Chemical Society
Pages: - Volume / Issue: 33 (21) Sequence Number: - Start / End Page: 8343 - 8350 Identifier: ISSN: 0897-4756
CoNE: https://pure.mpg.de/cone/journals/resource/954925561571