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Free keywords:
Condensed Matter, Superconductivity, cond-mat.supr-con, Condensed Matter, Strongly Correlated Electrons, cond-mat.str-el
Abstract:
Recent experiments in the doped cuprates La2−xBaxCuO4 have revealed the emission of anomalous terahertz radiation after impulsive optical excitation. The spectrum of this emission is sharply peaked in frequency at the Josephson plasma resonance. Notably, a prerequisite to this effect is that both superconducting and charge orders are present simultaneously. Here, we theoretically investigate the nonlinear electrodynamics of such striped superconductors and explore the origin of the observed radiation. We argue that photoexcitation is converted into a shift current by a second-order optical nonlinearity, which is activated by the breaking of inversion symmetry in certain stripe configurations. While such a low-frequency current impulsively drives both bulk and surface collective modes, we demonstrate that the observed emission is dominated by oscillations of the surface Josephson plasmon. Typically, surface excitations lie outside the light cone and are therefore silent; however, they can become bright due to the Bragg scattering off the charge order. We point out the importance of including Umklapp shift currents modulated at the stripe periodicity itself, which impulsively drive surface Josephson plasmons and lead to a resonant structure of outgoing radiation, consistent with the experiments.
