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  Gas-phase coupling in the CO oxidation reaction on polycrystalline platinum

Lauterbach, J., & Rotermund, H.-H. (1994). Gas-phase coupling in the CO oxidation reaction on polycrystalline platinum. Catalysis Letters, 27, 27-32. doi:10.1007/BF00806974.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0009-A21E-F Version Permalink: https://hdl.handle.net/21.11116/0000-0009-A5CC-7
Genre: Journal Article

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 Creators:
Lauterbach, Jochen1, Author           
Rotermund, Harm-Hinrich2, Author           
Affiliations:
1Fritz Haber Institute, Max Planck Society, ou_24021              
2Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              

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 Abstract: We report on self-sustained rate oscillations during the catalytic CO oxidation reaction on polycrystalline platinum. The photoelectron emission microscope enabled us to distinguish between three different types of grains. We found that the (110)- and the (100)-type grains are responsible for the development of rate oscillations while the (111)-type grains remain in a steady state. Gas-phase coupling is the dominant mechanism leading to a synchronisation of the different oscillating grains over macroscopic distances.

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Language(s): eng - English
 Dates: 1994-04-221994-05-051994-03
 Publication Status: Issued
 Pages: 6
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1007/BF00806974
 Degree: -

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Title: Catalysis Letters
  Abbreviation : Catal. Letters
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: New York : Springer
Pages: 6 Volume / Issue: 27 Sequence Number: - Start / End Page: 27 - 32 Identifier: ISSN: 1011-372X
CoNE: https://pure.mpg.de/cone/journals/resource/954925586300