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  Instrumentation for Hydrogenative Parahydrogen-Based Hyperpolarization Techniques

Schmidt, A., Bowers, C., Buckenmaier, K., Chekmenev, E., de Maissin, H., Eills, J., et al. (2022). Instrumentation for Hydrogenative Parahydrogen-Based Hyperpolarization Techniques. Analytical Chemistry, 94(1), 479-502. doi:10.1021/acs.analchem.1c04863.

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Schmidt, AB, Author
Bowers, CR, Author
Buckenmaier, K1, 2, Author              
Chekmenev, EY, Author
de Maissin, H, Author
Eills, J, Author
Ellermann, F, Author
Glöggler, S, Author
Gordon, JW, Author
Knecht, S, Author
Koptyug, IV, Author
Kuhn, J, Author
Pravdivtsev, AN, Author
Reineri, F, Author
Theis, T, Author
Them, K, Author
Hövener, J-B, Author
Affiliations:
1Department High-Field Magnetic Resonance, Max Planck Institute for Biological Cybernetics, Max Planck Society, ou_1497796              
2Max Planck Institute for Biological Cybernetics, Max Planck Society, Spemannstrasse 38, 72076 Tübingen, DE, ou_1497794              

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 Abstract: The unique properties of the entangled, antisymmetric nuclear spin state of dihydrogen, parahydrogen (pH2), has intrigued physicists, chemists, and other scientists for almost a century. pH2 was used as a model system in the early days of quantum mechanics (1) and is used for fueling rockets as well as combustion-free cars today. In the 1980s, pH2 was discovered as a convenient and potent source of spin order, allowing the enhancement of the signals of magnetic resonance (MR) by several orders of magnitude. (2−4) In the advent of hyperpolarized (HP) contrast agents (CA) for biomedical MR imaging (MRI) that followed, pH2-based hyperpolarization methods played an important role in the acquisition of the first HP 13C in vivo images (Figure 1). (5,6) Ever since, pH2 has proven to be highly valuable for analytical investigations and fundamental research, e.g., in analytical and catalytic chemistry or in the physics of singlet spin states. (7−10).

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 Dates: 2022-012022-01
 Publication Status: Published in print
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 Identifiers: DOI: 10.1021/acs.analchem.1c04863
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Title: Analytical Chemistry
  Abbreviation : Anal. Chem.
Source Genre: Journal
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Publ. Info: Washington, D.C. : American Chemical Society
Pages: - Volume / Issue: 94 (1) Sequence Number: - Start / End Page: 479 - 502 Identifier: ISSN: 0003-2700
CoNE: https://pure.mpg.de/cone/journals/resource/111032812862552