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  Highly selective population of spin-orbit levels in electronic autoionization of O2

Guyon, P.-M., Hepburn, J. W., Weng, T., Heiser, F., & Reynolds, D. (1991). Highly selective population of spin-orbit levels in electronic autoionization of O2. Physical Review Letters, 67(6), 675-678. doi:10.1103/PhysRevLett.67.675.

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Item Permalink: https://hdl.handle.net/21.11116/0000-0009-F5CA-F Version Permalink: https://hdl.handle.net/21.11116/0000-000A-12EA-A
Genre: Journal Article

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PhysRevLett.67.675.pdf (Publisher version), 207KB
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1991
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 Creators:
Guyon, Paul-Marie1, Author
Hepburn, John W.1, Author
Weng, Taimeng2, Author
Heiser, Franz3, Author           
Reynolds, David4, Author
Affiliations:
1Laboratoire des Collisions, Atomiques et Moléculaires, Université Paris XI, Bâtiment 351, 91405 Orsay, France, ou_persistent22              
2Laboratoire pour l’Utilisation, du Rayonnement Electromagnétique, Université Paris XI, Bâtiment 2090, 91405 Orsay, CEDEX France, ou_persistent22              
3Fritz Haber Institute, Max Planck Society, ou_24021              
4Department of Chemistry, University of Nottingham, Nottingham, United Kingdom, ou_persistent22              

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 Abstract: The dynamics of electronic autoionization in O2 has been studied using a new apparatus which combines a free-jet supersonic expansion with synchrotron radiation. Ions and electrons were analyzed by a double time-of-flight spectrometer. The spin-orbit sublevels of the 3Πu (v=0 and 2) Rydberg states in O2 were selectively excited and the resulting O+2 final states were determined by time-of-flight photoelectron spectros copy. A strong variation of the 2Π1/2g :2Π3/2g branching ratio was observed. This variation results from the selection of a single continuum wave function in the autoionization process.

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Language(s): eng - English
 Dates: 1991-03-251991-08-05
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.67.675
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: 4 Volume / Issue: 67 (6) Sequence Number: - Start / End Page: 675 - 678 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1