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  Mn (II) sub-nanometric sites stabilization in noble, N-doped carbonaceous materials for electrochemical CO2 reduction

Kossmann, J., Ortíz Sánchez-Manjavacas, M. L., Brandt, J., Heil, T., Lopez Salas, N., & Albero, J. (2022). Mn (II) sub-nanometric sites stabilization in noble, N-doped carbonaceous materials for electrochemical CO2 reduction. Chemical Communications, 58(31), 4841-4844. doi:10.1039/D2CC00585A.

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 Creators:
Kossmann, Janina1, Author              
Ortíz Sánchez-Manjavacas, María Luz1, Author
Brandt, Jessica2, Author              
Heil, Tobias2, Author              
Lopez Salas, Nieves1, Author              
Albero , Josep1, Author
Affiliations:
1Nieves Lopez Salas, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_3029702              
2Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863288              

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 Abstract: The preparation of stable and efficient electrocatalysts comprising abundant and non-critical row-materials is of paramount importance for its industrial implementation. Herein, we present a simple synthetic route to prepare Mn(II) sub-nanometric active sites over a highly N-doped noble carbonaceous support. This support not only promotes a strong stabilization of the Mn (II) sites, improving its stability against oxidation, but also provides a convenient coordination environment in the Mn (II) sites able to produce CO, HCOOH and CH3COOH from the electrochemically CO2 reduction.

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Language(s): eng - English
 Dates: 2022-03-212022
 Publication Status: Published in print
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 Identifiers: DOI: 10.1039/D2CC00585A
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Title: Chemical Communications
  Abbreviation : Chem. Commun.
Source Genre: Journal
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Publ. Info: Cambridge, UK : Royal Society of Chemistry
Pages: - Volume / Issue: 58 (31) Sequence Number: - Start / End Page: 4841 - 4844 Identifier: ISSN: 1359-7345