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  Rapid extraction of short-lived isotopes from a buffer gas cell for use in gas-phase chemistry experiments. Part I: Off-line studies with 219Rn and 221Fr

Goetz, S., Raeder, S., Block, M., Duellmann, C. E., Goetz, M., Jaeger, E., et al. (2021). Rapid extraction of short-lived isotopes from a buffer gas cell for use in gas-phase chemistry experiments. Part I: Off-line studies with 219Rn and 221Fr. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, 995: 165090. doi:10.1016/j.nima.2021.165090.

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 Urheber:
Goetz, S.1, Autor
Raeder, S.1, Autor
Block, M.1, Autor
Duellmann, Ch. E.1, Autor
Goetz, M.1, Autor
Jaeger, E.1, Autor
Kaleja, O.2, Autor           
Krier, J.1, Autor
Lens, L.1, Autor
Mistry, A. K.1, Autor
Mokry, Ch.1, Autor
Runke, J.1, Autor
Thoerle-Pospiech, P.1, Autor
Yakushev, A.1, Autor
Affiliations:
1external, ou_persistent22              
2Division Prof. Dr. Klaus Blaum, MPI for Nuclear Physics, Max Planck Society, ou_904548              

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 MPINP: Speichertechnik - Abteilung Blaum
 Zusammenfassung: To study the chemical properties of the heaviest elements, a fast and
efficient stopping and extraction of the highly energetic residues from
heavy ion fusion reactions into the chemistry setup is essential.
Currently used techniques like Recoil Transfer Chambers (RTC) relying on
gas flow extraction provide high efficiencies for chemically
non-reactive volatile species, but operate at extraction times t(extr)
of about 0.5 s or more. Buffer Gas Cells (BGC) with electric and
Radio-Frequency (RF) fields offer much faster extraction times. Here, we
demonstrate the successful coupling of a BGC to a gas chromatography
setup as is used for studies of chemical properties of superheavy
elements. Using Ra-223 and Ac-225 recoil ion sources providing Rn-219
and Fr-221 ions for off-line tests, an extraction time t(extr) = 55(4)
ms and an extraction efficiency of 35(3)% were achieved for the
non-reactive Rn-219, while Fr-221 was retained. The results show a
BGC-based setup to be suitable for gas-phase experiments with
short-lived volatile transactinide elements like Cn and Fl with
half-lives substantially below 1 s.

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 Datum: 2021-04-11
 Publikationsstatus: Online veröffentlicht
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 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: -
 Identifikatoren: ISI: 000694860700020
DOI: 10.1016/j.nima.2021.165090
 Art des Abschluß: -

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Titel: Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment
Genre der Quelle: Zeitschrift
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: Amsterdam : Elsevier B.V.
Seiten: - Band / Heft: 995 Artikelnummer: 165090 Start- / Endseite: - Identifikator: ISSN: 0168-9002
CoNE: https://pure.mpg.de/cone/journals/resource/954925485716