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  Controlling Floquet states on ultrashort time scales

Lucchini, M., Medeghini, F., Wu, Y., Vismarra, F., Borrego-Varillas, R., Crego, A., et al. (2022). Controlling Floquet states on ultrashort time scales. Nature Communications, 13(1): 7103. doi:10.1038/s41467-022-34973-4.

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Creators

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 Creators:
Lucchini, M.1, 2, Author
Medeghini, F.1, Author
Wu, Y.1, 2, Author
Vismarra, F.1, 2, Author
Borrego-Varillas, R.2, Author
Crego, A.2, Author
Frassetto, F.3, Author
Poletto, Luca3, Author
Sato, S.4, 5, Author           
Hübener, H.5, Author           
de Giovannini, U.5, 6, Author           
Rubio, A.5, 7, Author           
Nisoli, M.1, 2, Author
Affiliations:
1Department of Physics, Politecnico di Milano, ou_persistent22              
2Institute for Photonics and Nanotechnologies, IFN-CNR, 20133 Milano, ou_persistent22              
3Institute for Photonics and Nanotechnologies, IFN-CNR, 35131 Padova, ou_persistent22              
4Center for Computational Sciences, University of Tsukuba, ou_persistent22              
5Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
6Università degli Studi di Palermo, Dipartimento di Fisica e Chimica-Emilio Segrè, ou_persistent22              
7Center for Computational Quantum Physics (CCQ), The Flatiron Institute, ou_persistent22              

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Free keywords: Physics, Optics, physics.optics,physics.app-ph
 Abstract: The advent of ultrafast laser science offers the unique opportunity to combine Floquet engineering with extreme time resolution, further pushing the optical control of matter into the petahertz domain. However, what is the shortest driving pulse for which Floquet states can be realised remains an unsolved matter, thus limiting the application of Floquet theory to pulses composed by many optical cycles. Here we ionized Ne atoms with few-femtosecond pulses of selected time duration and show that a Floquet state can be observed already with a driving field that lasts for only 10 cycles. For shorter pulses, down to 2 cycles, the finite lifetime of the driven state can still be explained using an analytical model based on Floquet theory. By demonstrating that the amplitude and number of Floquet-like sidebands in the photoelectron spectrum can be controlled not only with the driving laser pulse intensity and frequency, but also by its duration, our results add a new lever to the toolbox of Floquet engineering.

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Language(s): eng - English
 Dates: 2022-05-062022-11-142022-11-19
 Publication Status: Published online
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: arXiv: 2205.00788
DOI: 10.1038/s41467-022-34973-4
 Degree: -

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Project name : -
Grant ID : 848411
Funding program : Horizon 2020 (H2020)
Funding organization : European Commission (EC)
Project name : This project has received funding from the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation program (grant agreement No. 848411 title AuDACE). M.L. and L.P. further acknowledge funding from MIUR PRIN aSTAR, Grant No. 2017RKWTMY. A.G. and R.B.-V. received funding from the DINAMO project funded by Fondazione Cariplo (grant no. 2020-4380). S.A.S., H.H., U.D.G., and A.R. were supported by the European Research Council (ERC-2015-AdG-694097) and Grupos Consolidados UPV/EHU (IT1249-19).
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Source 1

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Title: Nature Communications
  Abbreviation : Nat. Commun.
Source Genre: Journal
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Affiliations:
Publ. Info: London : Nature Publishing Group
Pages: - Volume / Issue: 13 (1) Sequence Number: 7103 Start / End Page: - Identifier: ISSN: 2041-1723
CoNE: https://pure.mpg.de/cone/journals/resource/2041-1723