English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT
  Application of an event-based camera for real-time velocity resolved kinetics

Golibrzuch, K., Schwabe, S., Zhong, T., Papendorf, K., & Wodtke, A. M. (2022). Application of an event-based camera for real-time velocity resolved kinetics. The Journal of Physical Chemistry A, 126(13), 2142-2148. doi:10.1021/acs.jpca.2c00806.

Item is

Files

show Files
hide Files
:
3384048.pdf (Publisher version), 3MB
Name:
3384048.pdf
Description:
-
OA-Status:
Hybrid
Visibility:
Public
MIME-Type / Checksum:
application/pdf / [MD5]
Technical Metadata:
Copyright Date:
-
Copyright Info:
-

Locators

show

Creators

show
hide
 Creators:
Golibrzuch, K.1, Author           
Schwabe, S.1, Author           
Zhong, T.1, Author           
Papendorf, K.1, Author           
Wodtke, A. M.1, Author           
Affiliations:
1Department of Dynamics at Surfaces, Max Planck Institute for Multidisciplinary Sciences, Max Planck Society, ou_3350158              

Content

show
hide
Free keywords: Physical Chemistry
 Abstract: We describe here the application of an inexpensive event-based/neuromorphic camera in an ion imaging experiment
operated at 1 kHz detection rate to study real-time velocity-resolved kinetics of thermal desorption. Such measurements involve a single gas pulse to initiate a time-dependent desorption process and a high repetition rate laser, where each pulse of the laser is used to produce an ion image. The sequence of ion images allows the time dependence of the desorption flux to be followed in real time. In previous work where a conventional framing camera was used, the large number of megapixel-sized images required data transfer and storage rates of up to 16 GB/s. This necessitated a large onboard memory that was quickly filled and limited continuous measurement to only a few seconds. Read-out of the memory became the bottleneck to the rate of data acquisition. We show here that since most pixels in each ion image contain no
data, the data rate can be dramatically reduced by using an event-based/neuromorphic camera. The data stream is thus reduced to the intensity and location information on the pixels that are lit up by each ion event together with a time-stamp indicating the arrival time of an ion at the detector. This dramatically increases the duty cycle of the method and provides insights for the execution of other high rep-rate ion imaging experiments.

Details

show
hide
Language(s): eng - English
 Dates: 2022-02-022022-03-232022-04-07
 Publication Status: Issued
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/acs.jpca.2c00806
 Degree: -

Event

show

Legal Case

show

Project information

show

Source 1

show
hide
Title: The Journal of Physical Chemistry A
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: -
Pages: - Volume / Issue: 126 (13) Sequence Number: - Start / End Page: 2142 - 2148 Identifier: -