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  Application of an event-based camera for real-time velocity resolved kinetics

Golibrzuch, K., Schwabe, S., Zhong, T., Papendorf, K., & Wodtke, A. M. (2022). Application of an event-based camera for real-time velocity resolved kinetics. The Journal of Physical Chemistry A, 126(13), 2142-2148. doi:10.1021/acs.jpca.2c00806.

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Golibrzuch, K.1, Autor           
Schwabe, S.1, Autor           
Zhong, T.1, Autor           
Papendorf, K.1, Autor           
Wodtke, A. M.1, Autor           
Affiliations:
1Department of Dynamics at Surfaces, Max Planck Institute for Multidisciplinary Sciences, Max Planck Society, ou_3350158              

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Schlagwörter: Physical Chemistry
 Zusammenfassung: We describe here the application of an inexpensive event-based/neuromorphic camera in an ion imaging experiment
operated at 1 kHz detection rate to study real-time velocity-resolved kinetics of thermal desorption. Such measurements involve a single gas pulse to initiate a time-dependent desorption process and a high repetition rate laser, where each pulse of the laser is used to produce an ion image. The sequence of ion images allows the time dependence of the desorption flux to be followed in real time. In previous work where a conventional framing camera was used, the large number of megapixel-sized images required data transfer and storage rates of up to 16 GB/s. This necessitated a large onboard memory that was quickly filled and limited continuous measurement to only a few seconds. Read-out of the memory became the bottleneck to the rate of data acquisition. We show here that since most pixels in each ion image contain no
data, the data rate can be dramatically reduced by using an event-based/neuromorphic camera. The data stream is thus reduced to the intensity and location information on the pixels that are lit up by each ion event together with a time-stamp indicating the arrival time of an ion at the detector. This dramatically increases the duty cycle of the method and provides insights for the execution of other high rep-rate ion imaging experiments.

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Sprache(n): eng - English
 Datum: 2022-02-022022-03-232022-04-07
 Publikationsstatus: Erschienen
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 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1021/acs.jpca.2c00806
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Titel: The Journal of Physical Chemistry A
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: -
Seiten: - Band / Heft: 126 (13) Artikelnummer: - Start- / Endseite: 2142 - 2148 Identifikator: -