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  Selective methane photooxidation into methanol under mild conditions promoted by highly dispersed Cu atoms on crystalline carbon nitrides

da Silva, M. A. R., Gil, J., Tarakina, N. V., Silva, G. T. S. T., Balena, J., Krambrock, K., et al. (2022). Selective methane photooxidation into methanol under mild conditions promoted by highly dispersed Cu atoms on crystalline carbon nitrides. Chemical Communications, 58(53), 7419-7422. doi:10.1039/D2CC01757A.

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 Creators:
da Silva, Marcos A R, Author
Gil, Jessica, Author
Tarakina, Nadezda V.1, Author              
Silva, Gelson T. S. T., Author
Balena, José, Author
Krambrock, Klaus, Author
Antonietti, Markus2, Author              
Ribeiro, Caue, Author
Teixeira, Ivo2, Author              
Affiliations:
1Nadezda V. Tarakina, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_2522693              
2Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society, ou_1863321              

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 Abstract: Here we report a photocatalytic system based on crystalline carbon nitrides (PHI) and highly dispersed transition metals (Fe, Co and Cu) for controlled methane photooxidation to methanol under mild conditions. The Cu-PHI catalyst showed a remarkable methanol production (2900 µmol.g-1) in 4 hours, with a turnover number of 51 moles of oxygenated liquid products per moles of Cu. Up to date, this result is the highest value for methane oxidation under mild conditions (1 bar, 25 °C).

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Language(s): eng - English
 Dates: 2022-05-312022
 Publication Status: Published in print
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 Identifiers: DOI: 10.1039/D2CC01757A
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Title: Chemical Communications
  Abbreviation : Chem. Commun.
Source Genre: Journal
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Publ. Info: Cambridge, UK : Royal Society of Chemistry
Pages: - Volume / Issue: 58 (53) Sequence Number: - Start / End Page: 7419 - 7422 Identifier: ISSN: 1359-7345