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  In-Situ Observation of the Formation of Laser-Induced Periodic Surface Structures with Extreme Spatial and Temporal Resolution

Sokolowski-Tinten, K., Bonse, J., Barty, A., Chapman, H. N., Bajt, S., Bogan, M. J., et al. (2023). In-Situ Observation of the Formation of Laser-Induced Periodic Surface Structures with Extreme Spatial and Temporal Resolution. In R. Stoian, & J. Bonse (Eds.), Ultrafast Laser Nanostructuring (Springer Series in Optical Sciences 239) (pp. 257-276). Springer Nature Switzerland AG. doi:10.1007/978-3-031-14752-4_6.

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978-3-031-14752-4_6.pdf (Publisher version), 2MB
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https://arxiv.org/abs/2206.04556 (Preprint)
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 Creators:
Sokolowski-Tinten, K.1, Author
Bonse, J.2, Author
Barty, A.3, Author
Chapman, H. N.4, 5, Author
Bajt, S.3, 6, Author
Bogan, M. J.7, Author
Boutet, S.8, Author
Cavalleri, A.9, Author           
Düsterer, S.3, Author
Frank, M.7, Author
Hajdu, J.10, 11, Author
Hau-Riege, S.7, Author
Marchesini, S.8, Author
Stojanovic, N.12, Author
Treusch, R.3, Author
Affiliations:
1Faculty of Physics and Centre for Nanointegration Duisburg-Essen, University of Duisburg-Essen, ou_persistent22              
2Bundesanstalt für Materialforschung und –prüfung (BAM), ou_persistent22              
3Deutsches Elektronen-Synchrotron DESY, ou_persistent22              
4Center for Free-Electron Laser Science, Deutsches Elektronen-Synchrotron DESY, ou_persistent22              
5Department of Physics and The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, ou_persistent22              
6The Hamburg Centre for Ultrafast Imaging, Universität Hamburg, ou_persistent22              
7Lawrence Livermore National Laboratory, ou_persistent22              
8SLAC National Accelerator Laboratory, ou_persistent22              
9Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938293              
10Department of Cell and Molecular Biology, Uppsala Universitet, ou_persistent22              
11he European Extreme Light Infrastructure, Institute of Physics, Academy of Sciences of the Czech Republic, ou_persistent22              
12Deutsches Zentrum für Luft- und Raumfahrt (DLR) , ou_persistent22              

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Free keywords: Laser-induced periodic surface structures (LIPSS), Capillary waves, Time-resolved scattering, Pump-probe experiments, Free electron laser
 Abstract: Irradiation of solid surfaces with intense ultrashort laser pulses represents a unique way of depositing energy into materials. It allows to realize states of extreme electronic excitation and/or very high temperature and pressure and to drive materials close to and beyond fundamental stability limits. As a consequence, structural changes and phase transitions often occur along unusual pathways and under strongly nonequilibrium conditions. Due to the inherent multiscale nature—both temporally and spatially—of these irreversible processes, their direct experimental observation requires techniques that combine high temporal resolution with the appropriate spatial resolution and the capability to obtain good quality data on a single pulse/event basis. In this respect, fourth-generation light sources, namely, short wavelength and short pulse free electron lasers (FELs), are offering new and fascinating possibilities. As an example, this chapter will discuss the results of scattering experiments carried out at the FLASH free electron laser at DESY (Hamburg, Germany), which allowed us to resolve laser-induced structure formation at surfaces on the nanometer to submicron length scale and in temporal regimes ranging from picoseconds to several nanoseconds with sub-picosecond resolution.

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Language(s): eng - English
 Dates: 2023-04-072023
 Publication Status: Issued
 Pages: 20
 Publishing info: -
 Table of Contents: -
 Rev. Type: Internal
 Identifiers: arXiv: 2206.04556
DOI: 10.1007/978-3-031-14752-4_6
ISBN: 978-3-031-14752-4
 Degree: -

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Project name : We are deeply indebted to Bruce Woods for his inventive engineering solutions that were critical for the success of these experiments, and his skill and efficiency in managing the construction of the instrumentation. We dedicate this to his memory. We also thank H. Ehrke, M. M. Seibert, and R. Tobey for their help during the experiment. This work was financially supported by the following agencies: the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) through the Collaborative Research Centre (CRC) 1242 (project number 278162697, project C01 Structural Dynamics in Impulsively Excited Nanostructures); the German Federal Ministry of Education and Research (FSP 301, grant 05KS7PG1); the US Department of Energy (DOE), Lawrence Livermore National Laboratory; the National Science Foundation Center for Biophotonics, University of California, Davis; the Advanced Light Source and National Centre for Electron Microscopy, Lawrence Berkeley National Laboratory, under contract DE-AC03-76SF00098; the Natural Sciences and Engineering Research Council of Canada (NSERC Postdoctoral Fellowship to M.J.B.); the Sven and Lilly Lawskis Foundation (doctoral fellowship to M.M.S.); the US Department of Energy Office of Science to the Stanford Linear Accelerator Center; the European Development Fund (structural dynamics of biomolecular systems—ELIBIO, CZ.02.1.01/0.0/0.0/15_003/0000447); the European Union (TUIXS); the Swedish Research Council; the Swedish Foundation for International Cooperation in Research and Higher Education; and the Swedish Foundation for Strategic Research. This work was performed under the auspices of the US DOE by Lawrence Livermore National Laboratory in part under contract W-7405-Eng-48 and in part under contract DE-AC52-07NA27344.
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Source 1

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Title: Ultrafast Laser Nanostructuring (Springer Series in Optical Sciences 239)
Source Genre: Book
 Creator(s):
Stoian, R.1, Editor
Bonse, J.2, Editor
Affiliations:
1 Laboratoire Hubert Curien, Université Jean Monnet, ou_persistent22            
2 Bundesanstalt für Materialforschung und -prüfung (BAM), ou_persistent22            
Publ. Info: Springer Nature Switzerland AG
Pages: - Volume / Issue: - Sequence Number: - Start / End Page: 257 - 276 Identifier: -