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  Sizes of pure and doped helium droplets from single shot x-ray imaging

Tanyag, R. M. P., Bacellar, C., Pang, W., Bernando, C., Gomez, L. F., Jones, C. F., et al. (2022). Sizes of pure and doped helium droplets from single shot x-ray imaging. The Journal of Chemical Physics, 156(4): 041102. doi:10.1063/5.0080342.

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Tanyag, Rico Mayro P.1, Autor
Bacellar, Camila1, Autor
Pang, Weiwu1, Autor
Bernando, Charles1, Autor
Gomez, Luis F.1, Autor
Jones, Curtis F.1, Autor
Ferguson, Ken R.1, Autor
Kwok, Justin1, Autor
Anielski , Denis1, Autor
Belkacem, Ali1, Autor
Boll, Rebecca2, Autor           
Bozek, John1, Autor
Carron, Sebastian1, Autor
Chen, Gang1, Autor
Delmas, Tjark1, Autor
Englert, Lars1, Autor
Epp, Sascha2, Autor           
Erk , Benjamin1, Autor
Foucar, Lutz1, Autor
Hartmann , Robert1, Autor
Hexemer, Alexander1, AutorHuth, Martin1, AutorLeone, Stephen R.1, AutorMa, Jonathan H.1, AutorMarchesini, Stefano1, AutorNeumark, Daniel M.1, AutorPoon, Billy K.1, AutorPrell, James1, AutorRolles, Daniel1, AutorRudek, Benedikt1, AutorRudenko, Artem1, AutorSeifrid, Martin1, AutorSwiggers, Michele1, AutorUllrich, Joachim1, AutorWeise, Fabian1, AutorZwart, Petrus1, AutorBostedt, Christoph1, AutorGessner, Oliver1, AutorVilesov, Andrey F.1, Autor mehr..
Affiliations:
1external, ou_persistent22              
2Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society, ou_2025284              

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 Zusammenfassung: Advancements in x-ray free-electron lasers on producing ultrashort, ultrabright, and coherent x-ray pulses enable single-shot imaging of fragile nanostructures, such as superfluid helium droplets. This imaging technique gives unique access to the sizes and shapes of individual droplets. In the past, such droplet characteristics have only been indirectly inferred by ensemble averaging techniques. Here, we report on the size distributions of both pure and doped droplets collected from single-shot x-ray imaging and produced from the free-jet expansion of helium through a 5 mu m diameter nozzle at 20 bars and nozzle temperatures ranging from 4.2 to 9 K. This work extends the measurement of large helium nanodroplets containing 10(9)-10(11) atoms, which are shown to follow an exponential size distribution. Additionally, we demonstrate that the size distributions of the doped droplets follow those of the pure droplets at the same stagnation condition but with smaller average sizes.

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 Datum: 2022-01-31
 Publikationsstatus: Online veröffentlicht
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 Ort, Verlag, Ausgabe: -
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 Art der Begutachtung: -
 Identifikatoren: DOI: 10.1063/5.0080342
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Titel: The Journal of Chemical Physics
  Kurztitel : J. Chem. Phys.
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: Woodbury, N.Y. : American Institute of Physics
Seiten: - Band / Heft: 156 (4) Artikelnummer: 041102 Start- / Endseite: - Identifikator: ISSN: 0021-9606
CoNE: https://pure.mpg.de/cone/journals/resource/954922836226