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  New electro-optic effect: Sum-frequency generation from optically active liquids in the presence of a dc electric field

Fischer, P., Buckingham, A. D., Beckwitt, K., Wiersma, D. S., & Wise, F. W. (2003). New electro-optic effect: Sum-frequency generation from optically active liquids in the presence of a dc electric field. Physical Review Letters, 91(17): 173901, pp. 173901-1-173901-4. doi:10.1103/PhysRevLett.91.173901.

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Item Permalink: https://hdl.handle.net/21.11116/0000-000A-F4A6-7 Version Permalink: https://hdl.handle.net/21.11116/0000-000A-F4A7-6
Genre: Journal Article

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PhysRevLett_91_2003_173901.pdf (Any fulltext), 166KB
 
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 Creators:
Fischer, Peer1, Author           
Buckingham, A. D., Author
Beckwitt, K., Author
Wiersma, D. S., Author
Wise, F. W., Author
Affiliations:
1Optical Nanoscopy, Max Planck Institute for Medical Research, Max Planck Society, ou_2364730              

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 Abstract: We report the observation of sum-frequency signals that depend linearly on an applied electrostatic field and that change sign with the handedness of an optically active solute. This recently predicted chiral electro-optic effect exists in the electric-dipole approximation. The static electric field gives rise to an electric-field-induced sum-frequency signal (an achiral third-order process) that interferes with the chirality-specific sum-frequency at second order. The cross-terms linear in the electrostatic field constitute the effect and may be used to determine the absolute sign of second- and third-order nonlinear-optical susceptibilities in isotropic media.

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Language(s): eng - English
 Dates: 2003-06-232003-10-24
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.91.173901
BibTex Citekey: ISI:000186138300019
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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: - Volume / Issue: 91 (17) Sequence Number: 173901 Start / End Page: 173901-1 - 173901-4 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1