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  Velocity map images of desorbing oxygen from sub-surface states of Rh(111)

Dorst, A., Güthoff, F., Schauermann, D., Wodtke, A. M., Killelea, D. R., & Schäfer, T. (2022). Velocity map images of desorbing oxygen from sub-surface states of Rh(111). Physical Chemistry Chemical Physics, 24, 26421-26427. doi:10.1039/D2CP03369K.

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Item Permalink: https://hdl.handle.net/21.11116/0000-000B-2AA5-C Version Permalink: https://hdl.handle.net/21.11116/0000-000C-D477-F
Genre: Journal Article

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 Creators:
Dorst, A.C.1, Author           
Güthoff, F.1, Author           
Schauermann, D., Author
Wodtke, A. M.1, Author                 
Killelea, Daniel R., Author
Schäfer, T.1, Author           
Affiliations:
1Department of Dynamics at Surfaces, Max Planck Institute for Multidisciplinary Sciences, Max Planck Society, Göttingen, DE, ou_3350158              

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 Abstract: We combine velocity map imaging (VMI) with temperature-programmed desorption (TPD) experiments to record the angular-resolved velocity distributions of recombinatively-desorbing oxygen from Rh(111). We assign the velocity distributions to desorption from specific surface and sub-surface states by matching the recorded distributions to the desorption temperature. These results provide insight into the recombinative desorption mechanisms and the availability of oxygen for surface-catalyzed reactions.

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Language(s): eng - English
 Dates: 2022-07-222022-09-092022
 Publication Status: Issued
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1039/D2CP03369K
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Title: Physical Chemistry Chemical Physics
Source Genre: Journal
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Pages: 7 Volume / Issue: 24 Sequence Number: - Start / End Page: 26421 - 26427 Identifier: ISSN: 1463-9076
ISSN: 1463-9084