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  Shedding New Light on Thermionic Electron Emission of Fullerenes

von Helden, G., Holleman, I., van Roij, A. J. A., Knippels, G. M. H., van der Meer, A. F. G., & Meijer, G. (1998). Shedding New Light on Thermionic Electron Emission of Fullerenes. Physical Review Letters, 81(9), 1825-1828. doi:10.1103/PhysRevLett.81.1825.

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Item Permalink: https://hdl.handle.net/21.11116/0000-000B-7882-B Version Permalink: https://hdl.handle.net/21.11116/0000-000B-7886-7
Genre: Journal Article

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PhysRevLett.81.1825.pdf (Publisher version), 178KB
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https://hdl.handle.net/21.11116/0000-000B-7884-9
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PhysRevLett.81.1825.pdf
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Copyright Date:
1998
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APS
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 Creators:
von Helden, G., Author
Holleman, I., Author
van Roij, A. J. A., Author
Knippels, G. M. H., Author
van der Meer, A. F. G., Author
Meijer, Gerard1, Author           
Affiliations:
1Department of Molecular and Laser Physics, University of Nijmegen, ou_persistent22              

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 Abstract: Tunable pulsed infrared (IR) radiation from a free electron laser is used to selectively excite fullerenes via their vibrational modes to very high internal energies. After absorbing several hundred IR photons, the molecules can autoionize. Ion creation is unexpectedly slow, occurring at times beyond 0.1 ms after laser excitation, but is found to be significantly faster for electronically preexcited molecules. It is concluded that reaching the first electronically excited state is a high hurdle on the way from hot molecules to ions.

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Language(s): eng - English
 Dates: 1998-02-251998-08-31
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.81.1825
 Degree: -

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Title: Physical Review Letters
  Abbreviation : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y. : American Physical Society
Pages: 4 Volume / Issue: 81 (9) Sequence Number: - Start / End Page: 1825 - 1828 Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1