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  Lowest Excited Singlet State of C60: A Vibronic Analysis of the Fluorescence

van den Heuvel, D. J., van den Berg, G. J. B., Groenen, E. J. J., Schmidt, J., Holleman, I., & Meijer, G. (1995). Lowest Excited Singlet State of C60: A Vibronic Analysis of the Fluorescence. The Journal of Physical Chemistry, 99(30), 11644-11649. doi:10.1021/j100030a004.

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 Creators:
van den Heuvel, D. J., Author
van den Berg, G. J. B., Author
Groenen, E. J. J., Author
Schmidt, J., Author
Holleman, I., Author
Meijer, Gerard1, Author           
Affiliations:
1Department of Molecular and Laser Physics, University of Nijmegen, ou_persistent22              

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 Abstract: The fluorescence and fluorescence-excitation spectra of C60 in a hydrocarbon glass at 1.2 K are reported.The fluorescence spectrum resembles that of a molecular X-trap in crystalline C60. The vibronic bands in these spectra are assigned, and the intensity distribution among the false origins points to vibronic coupling within the singlet manifold. The lowest excited singlet state of Cm shows predominantly T1g and G9 character. Additionally, we show that a reduction of the symmetry of C60 by either an intra- or an intermolecular perturbation leads to a fluorescence spectrum with a strong 0-0 transition and a different vibronic structure.

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Language(s): eng - English
 Dates: 1995-03-071995-07-01
 Publication Status: Issued
 Pages: 6
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/j100030a004
 Degree: -

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Title: The Journal of Physical Chemistry
  Abbreviation : J. Phys. Chem.
Source Genre: Journal
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Publ. Info: Washington, D.C. : American Chemical Society
Pages: 6 Volume / Issue: 99 (30) Sequence Number: - Start / End Page: 11644 - 11649 Identifier: ISSN: 1932-7447
CoNE: https://pure.mpg.de/cone/journals/resource/954926947766_3