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  Unified theoretical framework for mixing state of black carbon

Wang, J., Wang, J., Cai, R., Liu, C., Jiang, J., Nie, W., et al. (2022). Unified theoretical framework for mixing state of black carbon. EarthArXiv. doi:10.31223/X5C64D.

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 Creators:
Wang, Jiandong, Author
Wang, Jiaping, Author
Cai, Runlong, Author
Liu, Chao, Author
Jiang, Jingkun, Author
Nie, Wei, Author
Wang, Jinbo, Author
Moteki, Nobuhiro, Author
Zaveri, Rahul A., Author
Huang, Xin, Author
Ma, Nan, Author
Chen, Ganzhen, Author
Wang, Zilin, Author
Jin, Yuzhi, Author
Cai, Jing, Author
Zhang, Yuxuan, Author
Chi, Xuguang, Author
Holanda, Bruna1, Author           
Xing, Jia, Author
Liu, Tengyu, Author
Qi, Ximeng, AuthorWang, Qiaoqiao, AuthorPöhlker, Christopher1, Author           Su, Hang1, Author           Cheng, Yafang1, Author           Wang, Shuxiao, AuthorHao, Jiming, AuthorAndreae, Meinrat O.1, Author           Ding, Aijun, Author more..
Affiliations:
1Multiphase Chemistry, Max Planck Institute for Chemistry, Max Planck Society, ou_1826290              

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 Abstract: Black carbon (BC) plays an important role in the climate system due to its strong
warming effect, yet the magnitude of this effect is highly uncertain due to the complex mixing
state of aerosols. Here we build a unified theoretical framework to describe BC’s mixing states,
linking dynamic processes to BC coating thickness distribution, and show its self-similarity for
sites in diverse environments. The size distribution of BC-containing particles is found to follow
an exponential pattern and is independent of BC core size. A mixing state module is established
based on this finding and successfully applied in global and regional models, which increases the
accuracy of aerosol climate effect estimations. Our theoretical framework can bridge the gap be-
tween observation and model simulation in both mixing state description and light absorption quantification

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Language(s): eng - English
 Dates: 2022-08-312022-09
 Publication Status: Published online
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: No review
 Identifiers: DOI: 10.31223/X5C64D
 Degree: -

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Title: EarthArXiv
Source Genre: Journal
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