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  Spatially heterogeneous dynamics in a thermosensitive soft suspension before and after the glass transition

Colin, R., Alsayed, A. M., Castaing, J.-C., Goyal, R., Hough, L., & Abou, B. (2011). Spatially heterogeneous dynamics in a thermosensitive soft suspension before and after the glass transition. SOFT MATTER, 7(9), 4504-4514. doi:10.1039/c0sm01184c.

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アイテムのパーマリンク: https://hdl.handle.net/21.11116/0000-000B-C6D9-1 版のパーマリンク: https://hdl.handle.net/21.11116/0000-000C-14D6-C
資料種別: 学術論文

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 作成者:
Colin, Rémy1, 著者                 
Alsayed, Ahmed M.2, 著者
Castaing, Jean-Christophe2, 著者
Goyal, Rajesh2, 著者
Hough, Larry2, 著者
Abou, Berengere2, 著者
所属:
1Laboratoire Matière et Systèmes Complexes, UMR CNRS 7057, Université Paris Diderot, Paris, France, ou_persistent22              
2external, ou_persistent22              

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 要旨: The microscopic dynamics and aging of a soft thermosensitive suspension were investigated by looking at the thermal fluctuations of tracers in the suspension. Below and above the glass transition the dense microgel particle suspension was found to develop heterogeneous dynamics, characterized by a non Gaussian Probability Distribution Function (PDF) of the probes' displacements, with an exponential tail. We show that non Gaussian shapes are a characteristic of the ensemble-averaged PDF, while local PDFs remain Gaussian. This shows that the scenario behind the non Gaussian van Hove functions is a spatially heterogeneous dynamics, characterized by a spatial distribution of locally homogeneous dynamical environments through the sample, on the considered time scales. We characterize these statistical distributions of dynamical environments, in the liquid, supercooled, and glass states, and show that it can explain the exponential tail of the van Hove functions observed in the concentrated states. The intensity of spatial heterogeneities was found to amplify with increasing volume fraction. In the aging regime, it tends to increase as the glass gets more arrested.

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 日付: 2011
 出版の状態: 出版
 ページ: -
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 識別子(DOI, ISBNなど): ISI: 000289634000055
DOI: 10.1039/c0sm01184c
 学位: -

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出版物名: SOFT MATTER
種別: 学術雑誌
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ページ: - 巻号: 7 (9) 通巻号: - 開始・終了ページ: 4504 - 4514 識別子(ISBN, ISSN, DOIなど): ISSN: 1744-683X