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  Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems

Summers, A. M., Severino, S., Reduzzi, M., Sidiropoulos, T. P. H., Rivas, D. E., Di Palo, N., et al. (2023). Realizing Attosecond Core-Level X-ray Spectroscopy for the Investigation of Condensed Matter Systems. Ultrafast Science, 3: 0004. doi:10.34133/ultrafastscience.0004.

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Item Permalink: https://hdl.handle.net/21.11116/0000-000C-B6CE-F Version Permalink: https://hdl.handle.net/21.11116/0000-000C-E08C-9
Genre: Journal Article

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ultrafastscience.0004.pdf (Publisher version), 7MB
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Copyright Date:
2023
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© Adam M. Summers et al. Exclusive Licensee Xi’an Institute of Optics and Precision Mechanics. No claim to original U.S. Government Works.
License:
https://creativecommons.org/licenses/by/4.0/

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https://doi.org/10.34133/ultrafastscience.0004 (Publisher version)
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 Creators:
Summers, A. M.1, 2, Author
Severino, S.1, Author
Reduzzi, M.1, Author
Sidiropoulos, T. P. H.1, Author
Rivas, D. E.1, 3, Author
Di Palo, N.1, Author
Sun, H.-W.1, Author
Chien, Y.-H.1, Author
León, I.1, Author
Buades, B.1, Author
Cousin, S. L.1, Author
Teichmann, S. M.1, Author
Mey, T.4, Author
Mann, K.4, Author
Keitel, B.5, Author
Plönjes-Palm, E.5, Author
Efetov, D. K.1, Author
Schwoerer, H.6, Author           
Biegert, J.1, 7, Author
Affiliations:
1ICFO - Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, ou_persistent22              
2Linac Coherent Light Source, SLAC National Accelerator Laboratory, ou_persistent22              
3European XFEL, ou_persistent22              
4Institut für Nanophotonik Göttingen e.V. , ou_persistent22              
5Deutsches Elektronen-Synchrotron, ou_persistent22              
6Ultrafast Beams, Scientific Service Units, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_3255798              
7ICREA, ou_persistent22              

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 Abstract: Unraveling the exact nature of nonequilibrium and correlated interactions is paramount for continued progress in many areas of condensed matter science. Such insight is a prerequisite to develop an engineered approach for smart materials with targeted properties designed to address standing needs such as efficient light harvesting, energy storage, or information processing. For this goal, it is critical to unravel the dynamics of the energy conversion processes between carriers in the earliest time scales of the excitation dynamics. We discuss the implementation and benefits of attosecond soft x-ray core-level spectroscopy up to photon energies of 600 eV for measurements in solid-state systems. In particular, we examine how the pairing between coherent spectral coverage and temporal resolution provides a powerful new insight into the quantum dynamic interactions that determine the macroscopic electronic and optical response. We highlight the different building blocks of the methodology and point out the important aspects for its application from condensed matter studies to materials as thin as 25 nm. Furthermore, we discuss the technological developments in the field of tabletop attosecond soft x-ray sources with time-resolved measurements at the near and extended edge simultaneously and investigate the exciting prospective of extending such technique to the study of 2-dimensional materials.

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Language(s): eng - English
 Dates: 2022-08-142022-11-032023-03-312023-03
 Publication Status: Issued
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.34133/ultrafastscience.0004
 Degree: -

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Project name : J.B. acknowledges financial support from the European Research Council for ERC Advanced Grant “TRANSFORMER” (788218), ERC Proof of Concept Grant “miniX” (840010), FET-OPEN “PETACom” (829153), FET-OPEN “OPTOlogic” (899794), FET-OPEN “TwistedNano” (101046424), Laserlab-Europe (871124), Marie Skłodowska-Curie ITN “smart-X” (860553), MINECO for Plan Nacional PID2020–112664 GB-I00, AGAUR for 2017 SGR 1639, MINECO for “Severo Ochoa” (CEX2019-000910-S), Fundació Cellex Barcelona, the CERCA Programme/Generalitat de Catalunya, and the Alexander von Humboldt Foundation for the Friedrich Wilhelm Bessel Prize. S.S. acknowledges Marie Skłodowska-Curie grant agreement no. 713729 (COFUND). M.R. and A.M.S. acknowledge Marie Skłodowska-Curie Grant agreement no. 754510 (PROBIST).
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Title: Ultrafast Science
Source Genre: Journal
 Creator(s):
Affiliations:
Publ. Info: USA / China : AAAS / XIOPM (CAS)
Pages: - Volume / Issue: 3 Sequence Number: 0004 Start / End Page: - Identifier: ISSN: 2097-0331
ISSN: 2765-8791
CoNE: https://pure.mpg.de/cone/journals/resource/2097-0331